Release flux of heavy metals from river sediments at different flow rates

被引:10
作者
Lu, Jiangang [1 ,2 ]
Cai, Haisheng [1 ,3 ]
Zhang, Xueling [1 ]
Fu, Yanmei [4 ]
机构
[1] Jiangxi Agr Univ, Key Lab Po Yang Lake Watershed Agr Resources & Ec, Dev Res Ctr Selenium Rich Agr Ind, Nanchang 330045, Jiangxi, Peoples R China
[2] Jiangxi Water Resources Inst, Nanchang 330013, Jiangxi, Peoples R China
[3] Jiangxi Tourism & Commerce Vocat Coll, Nanchang 330100, Jiangxi, Peoples R China
[4] Yuzhang Normal Univ, Nanchang 330103, Jiangxi, Peoples R China
基金
中国国家自然科学基金;
关键词
flow rate; heavy metals; Le'an River; release flux; sediment; LEAN RIVER; DISSOLVED-OXYGEN; TRACE-METALS; WATER; PHOSPHORUS; LAKE; RESUSPENSION; TRANSPORT; SALINITY; ADSORPTION;
D O I
10.2166/ws.2021.251
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This paper simulates sediment motion under different hydrodynamic conditions, aiming to investigate the release flux of heavy metals in river sediments. During the lab experiments, carried out in a circular rectangular flume device, water velocity in the flume was altered by controlling the gate switch, and the flow rate was controlled from 0 to 1 m/s. Sediment from the Le'an River and chlorine-removed tap water were used as experimental sediment and water, respectively. Through analyses of Cu, Zn, Cd, and Pb concentration in water at different flow rates, the relationship between the release flux (y) of Cu, Zn, Cd, and Pb and the flow rate (x) was established with a fitting error of less than 15%. In order to judge the reliability of the conclusions, experimental results were verified outdoors. The results showed when the sediment particle size is between 0 and 250 mu m, within 1 hour, a quadratic polynomial correlation between the release flux of Cu, Cd, and Pb from river sediments and water velocity when the water pH is 5-9 and the flow rate is 0-65 cm/s; when the water pH is 5-9, the flow rate is 0-35 cm/s, the release flux of Zn from river sediments was shown to have a quadratic polynomial relationship with water velocity. The error between the calculated and measured values of heavy metals released from sediment in the Le'an River were within 5-30%. Our results can provide a theoretical reference for the control and treatment of heavy metal pollution in rivers and further improve corresponding water quality models.
引用
收藏
页码:542 / 554
页数:13
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