Integrated Photocatalytic Filtration Array for Indoor Air Quality Control

被引:34
作者
Denny, Frans [1 ]
Permana, Eric [1 ]
Scott, Jason [1 ]
Wang, Jing [2 ]
Pui, David Y. H. [2 ]
Amal, Rose [1 ]
机构
[1] Univ New S Wales, Sch Chem Engn, ARC Ctr Excellence Funct Nanomat, Sydney, NSW 2052, Australia
[2] Univ Minnesota, Dept Mech Engn, Particle Technol Lab, Minneapolis, MN 55455 USA
基金
澳大利亚研究理事会;
关键词
ORGANIC-COMPOUNDS; FILTER MEDIA; OXIDATION; TIO2; ETHANOL; NANOPARTICLES; 4-CHLOROPHENOL; PURIFICATION; DEGRADATION; WATER;
D O I
10.1021/es100421u
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Photocatalytic and filtration technologies were integrated to develop a hybrid system capable of removing and oxidizing organic pollutants from an air stream. A fluidized bed aerosol generator (FBAG) was adapted to prepare TiO2-loaded ventilation filters for the photodegradation of gas phase ethanol. Compared to a manually loaded filter, the ethanol photodegradation rate constant for the FBAG coated fitter increased by 361%. Additionally, the presence of the photogenerated intermediate product, acetaldehyde, was reduced and the time for mineralization to CO2 was accelerated. These improvements were attributed to the FBAG system providing a more uniform distribution of TiO2 particles across the filter surface leading to greater accessibility by the UV light A dual-UV-lamp system, as opposed to a single-lamp system, enhanced photocatalytic filter performance demonstrating the importance of high light irradiance and light distribution across the filter surface. Substituting the blacklight blue lamps with a UV-light-emitting-diode (UV-LED) array led to further improvement as well as suppressed the electrical energy per order (EE/O) by a factor of 6. These improvements derived from the more uniform distribution of light irradiance as well as the higher efficiency of UV-LEDs in converting electrical energy to photons.
引用
收藏
页码:5558 / 5563
页数:6
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