Enhanced magnetism in epitaxial SrRuO3 thin films

被引:67
作者
Grutter, Alexander [1 ,2 ]
Wong, Franklin [1 ]
Arenholz, Elke [3 ]
Liberati, Marco [3 ]
Vailionis, Arturas [4 ]
Suzuki, Yuri [1 ,2 ]
机构
[1] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA
[2] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA
[3] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA
[4] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA
关键词
ferromagnetic materials; internal stresses; magnetic epitaxial layers; magnetic moments; magnetisation; magnetomechanical effects; strontium compounds;
D O I
10.1063/1.3327512
中图分类号
O59 [应用物理学];
学科分类号
摘要
We observed enhanced magnetization in epitaxial SrRuO3 thin films compared to previously reported bulk and thin film values. The enhancement is strongly dependent on the orientation of the lattice distortions imposed by (001), (110), and (111) oriented SrTiO3 substrates. A larger magnetization enhancement for coherently strained SrRuO3 films on (111) and (110) oriented SrTiO3 compared to films on (001) SrTiO3 confirms the importance of the strain state in determining the magnetic ground state of the Ru ion. Moreover, SrRuO3 films on (111) SrTiO3 exhibit enhanced moments as high as 3.4 mu(B)/Ru ion, suggesting the stabilization of a high-spin Ru4+ state.
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页数:3
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共 14 条
[1]   Transport properties, thermodynamic properties, and electronic structure of SrRuO3 [J].
Allen, PB ;
Berger, H ;
Chauvet, O ;
Forro, L ;
Jarlborg, T ;
Junod, A ;
Revaz, B ;
Santi, G .
PHYSICAL REVIEW B, 1996, 53 (08) :4393-4398
[2]   SINGLE-CRYSTAL EPITAXIAL THIN-FILMS OF THE ISOTROPIC METALLIC OXIDES SR1-XCAXRUO3 (0-LESS-THAN-OR-EQUAL-TO-X-LESS-THAN-OR-EQUAL-TO-1) [J].
EOM, CB ;
CAVA, RJ ;
FLEMING, RM ;
PHILLIPS, JM ;
VANDOVER, RB ;
MARSHALL, JH ;
HSU, JWP ;
KRAJEWSKI, JJ ;
PECK, WF .
SCIENCE, 1992, 258 (5089) :1766-1769
[3]   Direct measurement of strain effects on magnetic and electrical properties of epitaxial SrRuO3 thin films [J].
Gan, Q ;
Rao, RA ;
Eom, CB ;
Garrett, JL ;
Lee, M .
APPLIED PHYSICS LETTERS, 1998, 72 (08) :978-980
[4]   Enhanced electron-electron correlations in nanometric SrRuO3 epitaxial films -: art. no. 174423 [J].
Herranz, G ;
Martínez, B ;
Fontcuberta, J ;
Sánchez, F ;
Ferrater, C ;
García-Cuenca, MV ;
Varela, M .
PHYSICAL REVIEW B, 2003, 67 (17)
[5]   HIGH-SPIN AND LOW-SPIN TRANSITION OF RU4+ IN THE PEROVSKITE-RELATED LAYERED SYSTEM SRN+1RUNO3N+1 (N=1, 2, AND INFINITY) WITH THE CHANGE IN N [J].
ITOH, M ;
SHIKANO, M ;
SHIMURA, T .
PHYSICAL REVIEW B, 1995, 51 (22) :16432-16435
[6]   Domain structure of epitaxial SrRuO3 thin films on miscut (001) SrTiO3 substrates [J].
Jiang, JC ;
Tian, W ;
Pan, XQ ;
Gan, Q ;
Eom, CB .
APPLIED PHYSICS LETTERS, 1998, 72 (23) :2963-2965
[7]   THE STRUCTURE OF SRRUO3 BY TIME-OF-FLIGHT NEUTRON POWDER DIFFRACTION [J].
JONES, CW ;
BATTLE, PD ;
LIGHTFOOT, P ;
HARRISON, WTA .
ACTA CRYSTALLOGRAPHICA SECTION C-CRYSTAL STRUCTURE COMMUNICATIONS, 1989, 45 :365-367
[8]   Tuning of magnetism in SrRuO3 thin films on SrTiO3 (001) substrate by control of the twin and strain amount in the buffer layer [J].
Lee, B. W. ;
Jung, C. U. ;
Kawasaki, M. ;
Tokura, Y. .
JOURNAL OF APPLIED PHYSICS, 2008, 104 (10)
[9]   Soft x-ray magnetic circular dichroism study of Ca1-xSrxRuO3 across the ferromagnetic quantum phase transition [J].
Okamoto, J. ;
Okane, T. ;
Saitoh, Y. ;
Terai, K. ;
Fujimori, S. -I. ;
Muramatsu, Y. ;
Yoshii, K. ;
Mamiya, K. ;
Koide, T. ;
Fujimori, A. ;
Fang, Z. ;
Takeda, Y. ;
Takano, M. .
PHYSICAL REVIEW B, 2007, 76 (18)
[10]   FAMILY OF O2- CENTERS IN SRO CRYSTALS [J].
SEEMAN, V ;
REIFMAN, S ;
LEHTO, T ;
HALDRE, U .
PHYSICA STATUS SOLIDI B-BASIC RESEARCH, 1980, 102 (02) :459-465