An extension of the Judd-Ofelt theory to the field of lanthanide thermometry

被引:60
作者
Ciric, Aleksandar [1 ]
Stojadinovic, Stevan [1 ]
Dramicanin, Miroslav D. [2 ]
机构
[1] Univ Belgrade, Fac Phys, Studentski Trg 12-16, Belgrade 11000, Serbia
[2] Univ Belgrade, Vinca Inst Nucl Sci, POB 522, Belgrade 11001, Serbia
关键词
Photoluminescence; Judd-ofelt; Lanthanide; Lminescence intensity ratio; Thermometry; THERMOGRAPHIC PHOSPHORS; SPECTRAL INTENSITIES; OPTICAL-ABSORPTION; ENERGY-TRANSFER; EU3+ IONS; TEMPERATURE; LUMINESCENCE; EMISSION; FLUORESCENCE; LIFETIME;
D O I
10.1016/j.jlumin.2019.116749
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
An extension of the Judd-Ofelt theory, a theoretical model to the field of Luminescence intensity ratio method in phosphor thermometry has been presented, that enables a calculation of thermometric figures of merit sensitivity, maximum sensitivity and temperature resolution, by the Judd-Ofelt intensity parameters. The model is applicable for 7 out of 14 lanthanides, and as a testing ground for the model's adequacy, Y2O3 doped with three different Eu3+ concentrations had been chosen. PL spectra were recorded up to 480 degrees C and photoluminescence and thermometric properties have been obtained. Conventionally estimated thermometric figures of merit have been compared to those obtained by a Judd-Ofelt thermometric model, with a good matching. Consequently, a novel method for calculation of magnetic dipole strength of the mixed induced electric dipole and magnetic dipole transition has been developed. Additionally, an interactive application software has been developed for the quick evaluation of the sensitivity and temperature resolution from Judd-Ofelt intensity parameters.
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页数:8
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