Direct observation of charge and orbital ordering in La0.5Sr1.5MnO4

被引:487
作者
Murakami, Y [1 ]
Kawada, H
Kawata, H
Tanaka, M
Arima, T
Moritomo, Y
Tokura, Y
机构
[1] High Energy Accelarator Res Org, Inst Mat Struct Sci, Photon Factory, Tsukuba, Ibaraki 3050801, Japan
[2] Univ Tsukuba, Inst Mat Sci, Tsukuba, Ibaraki 3050006, Japan
[3] Nagoya Univ, Ctr Integrated Res Sci & Engn, Nagoya, Aichi 4640814, Japan
[4] Univ Tokyo, Dept Appl Phys, Tokyo 1130033, Japan
[5] Joint Res Ctr Atom Technol, Tsukuba, Ibaraki 3050046, Japan
关键词
D O I
10.1103/PhysRevLett.80.1932
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Charge ordering and orbital ordering in La0.5Sr1.5MnO4 have been investigated by using synchrotron x-ray diffraction. The alternating pattern of Mn3+/Mn4+ in real space is observed directly by making use of their anomalous dispersion. The first clear evidence of the orbital ordering of e(g) electrons on Mn3+ is also presented based on the measurements of ATS (anisotropy of the tensor of susceptibility) reflection near the Mn K-absorption edge, The present observations indicate that the charge ordering and orbital ordering occur simultaneously at a transition temperature higher than that of the spin ordering.
引用
收藏
页码:1932 / 1935
页数:4
相关论文
共 25 条
[1]   A STRUCTURAL PHASE-TRANSITION INDUCED BY AN EXTERNAL MAGNETIC-FIELD [J].
ASAMITSU, A ;
MORITOMO, Y ;
TOMIOKA, Y ;
ARIMA, T ;
TOKURA, Y .
NATURE, 1995, 373 (6513) :407-409
[2]   Electronic phase separation and charge ordering in (Sr,La)(2)MnO4: Indication of triplet bipolarons [J].
Bao, W ;
Chen, CH ;
Carter, SA ;
Cheong, SW .
SOLID STATE COMMUNICATIONS, 1996, 98 (01) :55-59
[3]  
CHABARA K, 1993, APPL PHYS LETT, V63, P1990
[4]   CHARGE MODULATIONS IN LA2-XSRXNIO4+Y - ORDERING OF POLARONS [J].
CHEN, CH ;
CHEONG, SW ;
COOPER, AS .
PHYSICAL REVIEW LETTERS, 1993, 71 (15) :2461-2464
[5]   CHARGE-ORDERED STATES IN (LA,SR)2NIO4 FOR HOLE CONCENTRATIONS N(H)=1/3 AND N(H)=1/2 [J].
CHEONG, SW ;
HWANG, HY ;
CHEN, CH ;
BATLOGG, B ;
RUPP, LW ;
CARTER, SA .
PHYSICAL REVIEW B, 1994, 49 (10) :7088-7091
[6]   ANOMALOUS DISPERSION CALCULATIONS NEAR TO AND ON THE LONG-WAVELENGTH SIDE OF AN ABSORPTION-EDGE [J].
CROMER, DT ;
LIBERMAN, DA .
ACTA CRYSTALLOGRAPHICA SECTION A, 1981, 37 (MAR) :267-268
[7]   RELATIVISTIC CALCULATION OF ANOMALOUS SCATTERING FACTORS FOR X-RAYS [J].
CROMER, DT ;
LIBERMAN, D .
JOURNAL OF CHEMICAL PHYSICS, 1970, 53 (05) :1891-&
[8]   FORBIDDEN REFLECTIONS DUE TO ANISOTROPIC X-RAY SUSCEPTIBILITY OF CRYSTALS [J].
DMITRIENKO, VE .
ACTA CRYSTALLOGRAPHICA SECTION A, 1983, 39 (JAN) :29-35
[9]   THEORY OF THE ROLE OF COVALENCE IN THE PEROVSKITE-TYPE MANGANITES [LA,M(II)]MNO3 [J].
GOODENOUGH, JB .
PHYSICAL REVIEW, 1955, 100 (02) :564-573
[10]   THOUSANDFOLD CHANGE IN RESISTIVITY IN MAGNETORESISTIVE LA-CA-MN-O FILMS [J].
JIN, S ;
TIEFEL, TH ;
MCCORMACK, M ;
FASTNACHT, RA ;
RAMESH, R ;
CHEN, LH .
SCIENCE, 1994, 264 (5157) :413-415