Liquid hold-up and gas-liquid mass transfer in an alumina open-cell foam

被引:29
作者
Zapico, Rita R. [1 ]
Marin, Pablo [1 ]
Diez, Fernando V. [1 ]
Ordonez, Salvador [1 ]
机构
[1] Univ Oviedo, Fac Quim, Dept Chem & Environm Engn, Julian Claveria 8, Oviedo 33006, Spain
关键词
Reticulated structures; Phase contact; Trickle regime; Hold-up; Mass transfer coefficients; Heterogeneous reactors; MULTIPLE HYDRODYNAMIC STATES; COUNTER-CURRENT FLOW; SOLID FOAM; PRESSURE-DROP; HEAT-TRANSFER; TRICKLE FLOW; PACKED-BEDS; TRANSFER COEFFICIENT; SELECTIVE OXIDATION; METHANE COMBUSTION;
D O I
10.1016/j.ces.2016.01.008
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Open-cell foams are solid structures formed by an intricate network of macroporous interconnected channels. The high porosity and tortuosity of the channels results in high external surface area, so open cell foams are very efficient for promoting phase contact, e.g. in gas-liquid packed-bed reactors. In addition, the tortuous path of the channels breaks up the flow and enhances mass transfer with respect to other structured beds, such as honeycomb monoliths, and pressure drop is comparatively low. The liquid hold-up (system water-air), and the mass transfer coefficient (oxygen from water to nitrogen), have been measured for a ceramic foam, specifically a 20 ppi alumina foam bed of 50 mm diameter and 100 mm length (average pore diameter 1.25 mm and strut diameter 0.42 mm), for co-current down flow. Gas and liquid flow rates have been varied in the range corresponding to 0-8.5 . 10(-2) and 0-3.2 . 10(-3) m/s superficial velocities, respectively. At these conditions, the bed operates at trickle flow regime. The dynamic liquid hold-up and the mass transfer coefficient have been correlated as a function of relevant dimensionless numbers. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:297 / 304
页数:8
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