Emissions and treatment of VOCs emitted from wood-based construction materials: Impact on indoor air quality

被引:62
作者
Harb, P. [1 ]
Locoge, N. [1 ]
Thevenet, F. [1 ]
机构
[1] Univ Lille, SAGE, IMT Lille Douai, F-59000 Lille, France
关键词
Wood-based construction; VOC emission; Photocatalysis; Indoor air quality; PHOTOCATALYTIC OXIDATION; BUILDINGS; POLLUTION; PRODUCTS; BALANCE; HEALTH;
D O I
10.1016/j.cej.2018.08.085
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Concerns about insulation properties, bio-sourcing and recyclability of construction products promote the use of wood-based materials. Recent studies about indoor air quality in new constructions evidenced negative impacts of such material emissions on indoor air quality (IAQ). Efforts made on building air tightness to save energy promoted indoor pollutant confinement, encouraging the deployments of air treatment systems to improve IAQ. First, this study aims at characterizing wood-based material emissions in a real scale environment. Second, it aims at assessing the ability of widespread air treatment processes to address this specific IAQ problematic. Regarding emissions, a quantitative inventory of VOCs emitted by wood-based products is proposed. Terpenes and carbonyl VOCs (OVOCs) are the typical identified and quantified species. Concentration profiles of VOC and depletion rates are determined under environmental conditions. Then, the behaviors of two air treatment devices are addressed. It evidenced that the abatement of emitted VOCs not only depends on the chemical structure of the VOC but also on the conception of the device. Regarding terpenes, the devices induce noticeable but contrasted conversion rates. Moreover, possible sorption and transient secondary emissions of primary terpenes are evidenced. Regarding OVOCs, contrasted behaviors are observed between VOCs containing more than 4 carbon atoms compared to lighter ones. These behaviors still question the generation of lighter OVOCs as photocatalytic side-products, even in real scale environments. The proposed experimental approach gives a new insight and allows effective conclusions on sources and sinks of VOCs in a built environment.
引用
收藏
页码:641 / 652
页数:12
相关论文
共 29 条
[1]  
AFNOR, 2009, XPB44013 AFNOR
[2]  
[Anonymous], 2009, HIERARCHISATION SUBS
[3]  
[Anonymous], 2017, B OQAI
[4]   Indoor pollution and its impact on respiratory health [J].
Bardana, EJ .
ANNALS OF ALLERGY ASTHMA & IMMUNOLOGY, 2001, 87 (06) :33-40
[5]   VOCs and aldehydes source identification in European office buildings - The OFFICAIR study [J].
Campagnolo, Davide ;
Saraga, Dikaia E. ;
Cattaneo, Andrea ;
Spinazze, Andrea ;
Mandin, Corinne ;
Mabilia, Rosanna ;
Perreca, Erica ;
Sakellaris, Ioannis ;
Canha, Nuno ;
Mihucz, Victor G. ;
Szigeti, Tamas ;
Ventura, Gabriela ;
Madureira, Joana ;
Fernandes, Eduardo de Oliveira ;
de Kluizenaar, Yvonne ;
Cornelissen, Eric ;
Hanninen, Otto ;
Carrer, Paolo ;
Wolkoff, Peder ;
Cavallo, Domenico M. ;
Bartzis, John G. .
BUILDING AND ENVIRONMENT, 2017, 115 :18-24
[6]   VOC ternary mixture effect on ppb level photocatalytic oxidation: Removal kinetic, reaction intermediates and mineralization [J].
Debono, O. ;
Hequet, V. ;
Le Coq, L. ;
Locoge, N. ;
Thevenet, F. .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 218 :359-369
[7]   Gas phase photocatalytic oxidation of decane at ppb levels: Removal kinetics, reaction intermediates and carbon mass balance [J].
Debono, O. ;
Thevenet, F. ;
Gravejat, P. ;
Hequet, V. ;
Raillard, C. ;
Le Coq, L. ;
Locoge, N. .
JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2013, 258 :17-29
[8]   Toluene photocatalytic oxidation at ppbv levels: Kinetic investigation and carbon balance determination [J].
Debono, O. ;
Thevenet, F. ;
Gravejat, P. ;
Hequet, V. ;
Raillard, C. ;
Lecoq, L. ;
Locoge, N. .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2011, 106 (3-4) :600-608
[9]   The 40 m3 Innovative experimental Room for INdoor Air studies (IRINA): Development and validations [J].
Harb, P. ;
Sivachandiran, L. ;
Gaudion, V. ;
Thevenet, F. ;
Locoge, N. .
CHEMICAL ENGINEERING JOURNAL, 2016, 306 :568-578
[10]   Performance of ultraviolet photocatalytic oxidation for indoor air cleaning applications [J].
Hodgson, A. I. ;
Destaillats, H. ;
Sullivan, D. P. ;
Fisk, W. J. .
INDOOR AIR, 2007, 17 (04) :305-316