Manipulating twisted electrons in strong-field ionization

被引:23
作者
Maxwell, A. S. [1 ,2 ]
Armstrong, G. S. J. [3 ]
Ciappina, M. F. [2 ,4 ,5 ]
Pisanty, E. [2 ]
Kang, Y. [1 ]
Brown, A. C. [3 ]
Lewenstein, M. [2 ,6 ]
Figueira de Morisson Faria, C. [1 ]
机构
[1] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England
[2] Barcelona Inst Sci & Technol, ICFO Inst Ciencies Foton, Barcelona 08860, Spain
[3] Queens Univ Belfast, Sch Math & Phys, Ctr Theoret Atom Mol & Opt Phys, Univ Rd, Belfast BT7 1NN, Antrim, North Ireland
[4] Guangdong Technion Israel Inst Technol, Phys Program, Shantou 515063, Guangdong, Peoples R China
[5] Technion Israel Inst Technol, IL-32000 Haifa, Israel
[6] ICREA, Pg Lluis Co 23, Barcelona 08010, Spain
基金
英国工程与自然科学研究理事会;
关键词
ORBITAL ANGULAR-MOMENTUM; ABOVE-THRESHOLD IONIZATION; RECOIL-ION; VORTICES; PHOTOIONIZATION; LIGHT; PHOTOELECTRON; SPECTROSCOPY; MICROSCOPE; GENERATION;
D O I
10.1039/d0fd00105h
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We investigate the discrete orbital angular momentum (OAM) of photoelectrons freed in strong-field ionization. We use these 'twisted' electrons to provide an alternative interpretation on existing experimental work of vortex interferences caused by strong field ionization mediated by two counter-rotating circularly polarized pulses separated by a delay. Using the strong field approximation, we derive an interference condition for the vortices. In computations for a neon target we find very good agreement of the vortex condition with photoelectron momentum distributions computed with the strong field approximation, as well as with the time-dependent methods Qprop and R-Matrix. For each of these approaches we examine the OAM of the photoelectrons, finding a small number of vortex states localized in separate energy regions. We demonstrate that the vortices arise from the interference of pairs of twisted electron states. The OAM of each twisted electron state can be directly related to the number of arms of the spiral in that region. We gain further understanding by recreating the vortices with pairs of twisted electrons and use this to determine a semiclassical relation for the OAM. A discussion is included on measuring the OAM in strong field ionization directly or by employing specific laser pulse schemes as well as utilizing the OAM in time-resolved imaging of photo-induced dynamics.
引用
收藏
页码:394 / 412
页数:19
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