Lensfree OLEDs with over 50% external quantum efficiency via external scattering and horizontally oriented emitters

被引:105
作者
Song, Jinouk [1 ]
Kim, Kwon-Hyeon [2 ]
Kim, Eunhye [1 ]
Moon, Chang-Ki [2 ]
Kim, Yun-Hi [3 ,4 ]
Kim, Jang-Joo [2 ]
Yoo, Seunghyup [1 ]
机构
[1] Korea Adv Inst Sci & Technol, Sch Elect Engn, Daejeon 34141, South Korea
[2] Seoul Natl Univ, Dept Mat Sci & Engn, Seoul 151744, South Korea
[3] Gyeongsang Natl Univ, Dept Chem, Jinju 66701, South Korea
[4] Gyeongsang Natl Univ, ERI, Jinju 66701, South Korea
来源
NATURE COMMUNICATIONS | 2018年 / 9卷
基金
新加坡国家研究基金会;
关键词
D O I
10.1038/s41467-018-05671-x
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
High efficiency is important for successful deployment of any light sources. Continued efforts have recently made it possible to demonstrate organic light-emitting diodes with efficiency comparable to that of inorganic light-emitting diodes. However, such achievements were possible only with the help of a macroscopic lens or complex internal nanostructures, both of which undermine the key benefits of organic light-emitting diodes as an affordable planar light source. Here we present a systematic way to achieve organic light-emitting diodes with ultrahigh efficiency even only with an external scattering film, one of the simplest low-cost outcoupling structures. Through a global, multivariable analysis, we show that scattering with a high degree of forwardness has a potential to play a critical role in realizing ultimate efficiency. Combined with horizontally oriented emitters, organic light-emitting diodes equipped with particle-embedded films tailored for forward-intensive scattering achieve a maximum external quantum efficiency of 56%.
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页数:10
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  • [1] Adachi C., Baldo M.A., Thompson M.E., Forrest S.R., Nearly 100% internal phosphorescence efficiency in an organic light-emitting device, J. Appl. Phys., 90, pp. 5048-5051, (2001)
  • [2] Reineke S., Et al., White organic light-emitting diodes with fluorescent tube efficiency, Nature, 459, pp. 234-238, (2009)
  • [3] Uoyama H., Goushi K., Shizu K., Nomura H., Adachi C., Highly efficient organic light-emitting diodes from delayed fluorescence, Nature, 492, pp. 234-238, (2012)
  • [4] Gaj M.P., Fuentes-Hernandez C., Zhang Y., Marder S.R., Kippelen B., Highly efficient Organic Light-Emitting Diodes from thermally activated delayed fluorescence using a sulfone–carbazole host material, Org. Electron., 16, pp. 109-112, (2015)
  • [5] Liu X.K., Et al., Remanagement of singlet and triplet excitons in single-emissive-layer hybrid white organic light-emitting devices using thermally activated delayed fluorescent blue Exciplex, Adv. Mater., 27, pp. 7079-7085, (2015)
  • [6] Seino Y., Inomata S., Sasabe H., Pu Y.J., Kido J., High-performance green OLEDs using thermally activated delayed fluorescence with a power efficiency of over 100 lm W<sup>−1</sup> , Adv. Mater., 28, pp. 2638-2643, (2016)
  • [7] Lin T.A., Et al., Sky-blue organic light emitting diode with 37% external quantum efficiency using thermally activated delayed fluorescence from spiroacridine-triazine hybrid, Adv. Mater., 28, pp. 6976-6983, (2016)
  • [8] Gather M.C., Reineke S., Recent advances in light outcoupling from white organic light-emitting diodes, J. Photonics Energy, 5, (2015)
  • [9] Moller S., Forrest S.R., Improved light out-coupling in organic light emitting diodes employing ordered microlens arrays, J. Appl. Phys., 91, pp. 3324-3327, (2002)
  • [10] Chang H.W., Et al., Nano-particle based scattering layers for optical efficiency enhancement of organic light-emitting diodes and organic solar cells, J. Appl. Phys., 113, (2013)