The effect of chemical vapor deposition temperature on the performance of binder-free sewage sludge-derived anodes in microbial fuel cells

被引:32
作者
Feng, Huajun
Jia, Yufeng
Shen, Dongsheng
Zhou, Yuyang
Chen, Ting
Chen, Wei
Ge, Zhipeng
Zheng, Shuting
Wang, Meizhen
机构
[1] Zhejiang Gongshang Univ, Sch Environm Sci & Engn, Hangzhou 310012, Zhejiang, Peoples R China
[2] Zhejiang Prov Key Lab Solid Waste Treatment & Rec, Hangzhou 310012, Zhejiang, Peoples R China
基金
中国国家自然科学基金;
关键词
Sewage sludge-derived anode; Carbonization temperature; Carbon micro-wires; Microbial fuel cells; Power density; ACTIVATED CARBON; BIOANODE;
D O I
10.1016/j.scitotenv.2018.04.124
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Conversion of sewage sludge (SS) into value-added material has garnered increasing attention due to its potential applications. In this study, we propose a new application of the sewage sludge-derived carbon (SSC) as an electrode without binder in microbial fuel cells (MFCs). SS was firstly converted into SSC monoliths by methane chemical vapormethod at different temperature (600, 800, 1000 or 1200 degrees C). Scanning electron microscopy images showed that carbon micro-wireswere present on the surfaces of the samples prepared at 1000 and 1200 degrees C. The results showed that it was beneficial for converting sludge into a highly conductive electrode and increasing carbon content of the electrode at higher temperatures, thereby improving the current generation. The conductivity results show that a higher temperature favors the conversion of sludge into a highly conductive electrode. TheMFC using an SSC anode processed at 1200 degrees C generated the maximumpower density of 2228mWm(-2) and the maximum current density of 14.2 A m(-2). This value was 5 times greater than that generated by an MFC equipped with a graphite anode. These results present a promising means of converting SS into electrode materials. (C) 2018 Elsevier B.V. All rights reserved.
引用
收藏
页码:45 / 52
页数:8
相关论文
共 32 条
[1]   Layered corrugated electrode macrostructures boost microbial bioelectrocatalysis [J].
Chen, Shuiliang ;
He, Guanghua ;
Liu, Qin ;
Harnisch, Falk ;
Zhou, Yan ;
Chen, Yu ;
Hanif, Muddasir ;
Wang, Suqin ;
Peng, Xinwen ;
Hou, Haoqing ;
Schroeder, Uwe .
ENERGY & ENVIRONMENTAL SCIENCE, 2012, 5 (12) :9769-9772
[2]   In Situ Electrochemically Derived Nanoporous Oxides from Transition Metal Dichalcogenides for Active Oxygen Evolution Catalysts [J].
Chen, Wei ;
Liu, Yayuan ;
Li, Yuzhang ;
Sun, Jie ;
Qiu, Yongcai ;
Liu, Chong ;
Zhou, Guangmin ;
Cui, Yi .
NANO LETTERS, 2016, 16 (12) :7588-7596
[3]   Capacitive Bioanodes Enable Renewable Energy Storage in Microbial Fuel Cells [J].
Deeke, Alexandra ;
Sleutels, Tom H. J. A. ;
Hamelers, Hubertus V. M. ;
Buisman, Cees J. N. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2012, 46 (06) :3554-3560
[4]   Anode modification with capacitive materials for a microbial fuel cell: an increase in transient power or stationary power [J].
Feng, Chunhua ;
Lv, Zhisheng ;
Yang, Xiaoshuang ;
Wei, Chaohai .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2014, 16 (22) :10464-10472
[5]   TiO2 Nanotube Arrays Modified Titanium: A Stable, Scalable, and Cost-Effective Bioanode for Microbial Fuel Cells [J].
Feng, Huajun ;
Liang, Yuxiang ;
Guo, Kun ;
Chen, Wei ;
Shen, Dongsheng ;
Huang, Lijie ;
Zhou, Yuyang ;
Wang, Meizhen ;
Long, Yuyang .
ENVIRONMENTAL SCIENCE & TECHNOLOGY LETTERS, 2016, 3 (12) :420-424
[6]   Mini-review: Anode modification for improved performance of microbial fuel cell [J].
Hindatu, Y. ;
Annuar, M. S. M. ;
Gumel, A. M. .
RENEWABLE & SUSTAINABLE ENERGY REVIEWS, 2017, 73 :236-248
[7]   Degradation and characteristic changes of organic matter in sewage sludge using microbial fuel cell with ultrasound pretreatment [J].
Jiang, Junqiu ;
Zhao, Qingliang ;
Wei, Liangliang ;
Wang, Kun ;
Lee, Duu-Jong .
BIORESOURCE TECHNOLOGY, 2011, 102 (01) :272-277
[8]   FORMATION AND REDUCTION OF NITROGEN-OXIDES IN FLUIDIZED-BED COMBUSTION [J].
JOHNSSON, JE .
FUEL, 1994, 73 (09) :1398-1415
[9]   Carbon Nanofiber/Polypyrrole Nanocomposite as Anode Material in Microbial Fuel Cells [J].
Jung, Ho-Young ;
Roh, Sung-Hee .
JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY, 2017, 17 (08) :5830-5833
[10]   Recent advances and challenges in the anode architecture and their modifications for the applications of microbial fuel cells [J].
Kumar, G. Gnana ;
Sarathi, V. G. Sathiya ;
Nahm, Kee Suk .
BIOSENSORS & BIOELECTRONICS, 2013, 43 :461-475