Optimization of catalyst distribution along PEMFC channel through a numerical two-phase model and genetic algorithm

被引:47
作者
Ebrahimi, Sasan [1 ]
Ghorbani, Babak [1 ]
Vijayaraghavan, Krishna [1 ]
机构
[1] Simon Fraser Univ, Sch Mechatron Syst Engn, 250-13450 102 Ave, Surrey, BC V3T 0A3, Canada
关键词
Optimum catalyst loading; PEMFC power density; Two-phase flow; Multiphase mixture model (M2); Non-uniform catalyst distribution; Genetic algorithm; ELECTROLYTE FUEL-CELLS; GAS-DIFFUSION LAYER; CATHODE; TRANSPORT; FLOW; MULTICOMPONENT; PERFORMANCE; GRADIENT; MEDIA; WATER;
D O I
10.1016/j.renene.2017.06.067
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this paper, a new approach is presented to find the optimum catalyst loading distribution along the flow field. The optimization is performed by integrating a computational fluid dynamic (CFD) model and genetic algorithm optimization method. The CFD model is two-dimensional, steady state and two-phase. Multiphase mixture model (M-2) is used to model two-phase transport in porous media of a Polymer Electrolyte Membrane Fuel Cell (PEMFC). Numerical domain includes channel, gas diffusion layer (GDL) and catalyst layer (CL) in the cathode side. In the next step, current density is assumed to be proportional with catalyst loading. Catalyst loading is considered as polynomial functions with unknown coefficients. Genetic algorithm optimization method is applied to find the unknown coefficients and as a result the optimum catalyst loading function along the flow field. The results indicate that catalyst loading distribution has a significant effect on the fuel cell performance and it is seen that in the optimum case, maximum PEMFC power density is increased by about 14%. (C)2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码:846 / 854
页数:9
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