Fluid modelling of a packed bed dielectric barrier discharge plasma reactor

被引:148
作者
Van Laer, Koen [1 ]
Bogaerts, Annemie [1 ]
机构
[1] Univ Antwerp, Dept Chem, Res Grp PLASMANT, Univ Pl 1, B-2610 Antwerp, Belgium
关键词
plasmas; dielectric barrier discharge; packing; modelling; ATMOSPHERIC-PRESSURE; ENERGY EFFICIENCY; OZONE SYNTHESIS; REMOVAL; HELIUM; SIMULATION; CONVERSION; CATALYSIS; GASES;
D O I
10.1088/0963-0252/25/1/015002
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
A packed bed dielectric barrier discharge plasma reactor is computationally studied with a fluid model. Two different complementary axisymmetric 2D geometries are used to mimic the intrinsic 3D problem. It is found that a packing enhances the electric field strength and electron temperature at the contact points of the dielectric material due to polarization of the beads by the applied potential. As a result, these contact points prove to be of direct importance to initiate the plasma. At low applied potential, the discharge stays at the contact points, and shows the properties of a Townsend discharge. When a high enough potential is applied, the plasma will be able to travel through the gaps in between the beads from wall to wall, forming a kind of glow discharge. Therefore, the inclusion of a so-called 'channel of voids' is indispensable in any type of packed bed modelling.
引用
收藏
页数:11
相关论文
共 38 条
[1]   Carbon Dioxide Splitting in a Dielectric Barrier Discharge Plasma: A Combined Experimental and Computational Study [J].
Aerts, Robby ;
Somers, Wesley ;
Bogaerts, Annemie .
CHEMSUSCHEM, 2015, 8 (04) :702-716
[2]  
[Anonymous], KINEMA RES SOFTWARE
[3]   Surface charge accumulation and discharge development in diffuse and filamentary barrier discharges operating in He, N2 and mixtures [J].
Bogaczyk, M. ;
Wild, R. ;
Stollenwerk, L. ;
Wagner, H-E .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2012, 45 (46)
[4]   Gas discharge plasmas and their applications [J].
Bogaerts, A ;
Neyts, E ;
Gijbels, R ;
van der Mullen, J .
SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2002, 57 (04) :609-658
[5]   Decomposition of toluene and acetone in packed dielectric barrier discharge reactors [J].
Chang, CL ;
Lin, TS .
PLASMA CHEMISTRY AND PLASMA PROCESSING, 2005, 25 (03) :227-243
[6]   Removal of NF3 from semiconductor-process flue gases by tandem packed-bed plasma and adsorbent hybrid systems [J].
Chang, JS ;
Kostov, KG ;
Urashima, K ;
Yamamoto, T ;
Okayasu, Y ;
Kato, T ;
Iwaizumi, T ;
Yoshimura, K .
IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, 2000, 36 (05) :1251-1259
[7]   Enhancement of energy yield for ozone production via packed-bed reactors [J].
Chen, HL ;
Lee, HM ;
Chang, MB .
OZONE-SCIENCE & ENGINEERING, 2006, 28 (02) :111-118
[8]   Review of packed-bed plasma reactor for ozone generation and air pollution control [J].
Chen, Hsin Liang ;
Lee, How Ming ;
Chen, Shiaw Huei ;
Chang, Moo Been .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2008, 47 (07) :2122-2130
[9]   Review of plasma catalysis on hydrocarbon reforming for hydrogen production-Interaction, integration, and prospects [J].
Chen, Hsin Liang ;
Lee, How Ming ;
Chen, Shiaw Huei ;
Chao, Yu ;
Chang, Moo Been .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2008, 85 (1-2) :1-9
[10]   Removal of formaldehyde from gas streams via packed-bed dielectric barrier discharge plasmas [J].
Ding, HX ;
Zhu, AM ;
Yang, XF ;
Li, CH ;
Xu, Y .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2005, 38 (23) :4160-4167