High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response

被引:199
作者
Thirimanne, H. M. [1 ]
Jayawardena, K. D. G. I. [1 ]
Parnell, A. J. [2 ]
Bandara, R. M. I. [1 ]
Karalasingam, A. [1 ]
Pani, S. [3 ]
Huerdler, J. E. [4 ]
Lidzey, D. G. [2 ]
Tedde, S. F. [4 ]
Nisbet, A. [3 ,5 ]
Mills, C. A. [1 ]
Silva, S. R. P. [1 ]
机构
[1] Univ Surrey, Adv Technol Inst, Dept Elect & Elect Engn, Guildford GU2 7XH, Surrey, England
[2] Univ Sheffield, Dept Phys & Astron, Hicks Bldg, Sheffield S3 7RH, S Yorkshire, England
[3] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England
[4] Technol Ctr, Siemens Healthineers GmbH, D-91058 Erlangen, Germany
[5] Royal Surrey Cty Hosp NHS Fdn Trust, Dept Med Phys, Egerton Rd, Guildford GU2 7XX, Surrey, England
基金
“创新英国”项目; 英国工程与自然科学研究理事会;
关键词
PEROVSKITE SINGLE-CRYSTALS; LEAD HALIDE PEROVSKITES; AMORPHOUS SELENIUM; ELECTRIC-FIELDS; SOLAR-CELLS; PHOTODETECTORS; PERFORMANCE; TRANSPORT; EMISSION; PHOTONS;
D O I
10.1038/s41467-018-05301-6
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
X-ray detectors are critical to healthcare diagnostics, cancer therapy and homeland security, with many potential uses limited by system cost and/or detector dimensions. Current X-ray detector sensitivities are limited by the bulk X-ray attenuation of the materials and consequently necessitate thick crystals (similar to 1 mm(-1) cm), resulting in rigid structures, high operational voltages and high cost. Here we present a disruptive, flexible, low cost, broadband, and high sensitivity direct X-ray transduction technology produced by embedding high atomic number bismuth oxide nanoparticles in an organic bulk heterojunction. These hybrid detectors demonstrate sensitivities of 1712 mu C mGy(-1) cm(-3) for "soft" X-rays and similar to 30 and 58 mu C mGy(-1) cm(-3) under 6 and 15 MV "hard" X-rays generated from a medical linear accelerator; strongly competing with the current solid state detectors, all achieved at low bias voltages (-10 V) and low power, enabling detector operation powered by coin cell batteries.
引用
收藏
页数:10
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