Structure and non-linear optical properties of BaO-TiO2-SiO2 glass containing Ba2TiSi2O8 crystal

被引:55
作者
Masai, Hirokazu
Tsuji, Shinji
Fujiwara, Takumi
Benino, Yasuhiko
Komatsu, Takayuki
机构
[1] Tohoku Univ, Dept Appl Phys, Aoba Ku, Sendai, Miyagi 9808579, Japan
[2] Nagaoka Univ Technol, Dept Mat Sci & Technol, Nagaoka, Niigata 9402188, Japan
关键词
glass ceramics; non-linear optics;
D O I
10.1016/j.jnoncrysol.2007.03.005
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The BaO TiO2-Sio(2) crystallized glass containing Ba2TiSi2O8 crystal phase was examined using X-ray diffraction (XRD) measurement and Maker fringe technique. It has been found that the crystallized glasses with a composition of close to the stoichiometric Ba2TiSi2O8 showed bulk crystallization, whereas other crystallized glasses with non-stoichiometric composition of Ba2TiSi2O8 showed surface crystallization. The parameter AT, the difference in temperature between the crystallization onset and the glass transition temperature, strongly affects the crystallization behaviors of the present BTS glasses. The 30BaO-20TiO(2)-50SiO(2) transparent surface crystallized glass with strong c-oriented BaTiSi2O8 phase showed its second-order non-linear optical constant, d(33) = 6.1 pm/V. (c) 2007 Published by Elsevier B.V.
引用
收藏
页码:2258 / 2262
页数:5
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