An industrial demonstration study on CO2 mineralization curing for concrete

被引:22
作者
Wang, Tao [1 ]
Yi, Zhenwei [1 ]
Song, Jiayi [1 ]
Zhao, Chao [2 ]
Guo, Ruonan [1 ]
Gao, Xiang [1 ]
机构
[1] Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou, Peoples R China
[2] Clean Carbon Beijing Technol Co Ltd, Beijing, Peoples R China
关键词
CARBONATION; SEQUESTRATION; TECHNOLOGIES; PERFORMANCE; WASTE; PASTE;
D O I
10.1016/j.isci.2022.104261
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
A 10,000 ton-CO2/y mineralization curing (CMC) process was demonstrated in Jiaozuo city, China by retrofitting a traditional autoclaved curing plant. An industrial concrete formula with synergistic effects of aggregate gradation, early hydration, and alkali excitation was developed using local solid wastes resources. Approximately 90% of the raw materials, including fly ash, furnace blaster slag, steel slag, and carbide slag, came from coal-based industries. An extraordinary phenomenon of high-temperature accumulation from room temperature to 140 degrees C was first observed in an industrial scale because of the rapid and strong exothermic carbonation reaction. A step pressure-equalizing procedure was developed to achieve a rapid carbonation rate, a high CO2 conversion ratio of >98%, and efficient carbonation exotherm recycling. The global warming potential life cycle analysis revealed that compared with autoclaved curing, CMC showed significantly decreased the emission of 182 kg CO2-Eq/m(3)-product, with direct CO2 sequestration accounting for similar to 65% of the reduction.
引用
收藏
页数:18
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