Strong-field spatiotemporal ultrafast coherent control in three-level atoms

Simple analytical approaches for implementing strong field coherent control schemes are often elusive due to the complexity of the interaction between the intense excitation field and the system of interest. Here, we demonstrate control over multiphoton excitation in a three-level resonant system using simple, analytically derived ultrafast pulse shapes. We utilize a two-dimensional spatiotemporal control technique, in which temporal focusing produces a spatially dependent quadratic spectral phase, while a second, arbitrary phase parameter is scanned using a pulse shaper. In the current work, we demonstrate weak-to-strong field excitation of Rb-85, with a pi phase step and the quadratic phase as the chosen control parameters. The intricate dependence of the multilevel dynamics on these parameters is exhibited by mapping the data onto a two-dimensional control landscape. Further insight is gained by simulating the complete landscape using a dressed-state, time-domain model, in which the influence of individual shaping parameters can be extracted using both exact and asymptotic time-domain representations of the dressed-state energies.