Two-photon-resonance four-wave mixing for the study of permanent molecular dipoles

被引：0
作者：
Hadjichristov, GB
Kirov, N
Materny, A
Kiefer, W
机构：
[1] Univ Wurzburg, Inst Phys Chem, D-97074 Wurzburg, Germany
[2] Inst Solid State Phys, BG-1784 Sofia, Bulgaria
来源：
JOURNAL OF RAMAN SPECTROSCOPY | 1998年 / 29卷 / 04期
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D O I：
暂无
中图分类号：
O433 [光谱学];
学科分类号：
0703 ; 070302 ;
摘要：
Two-photon-resonance four-wave mixing (TPR-FWM) spectroscopy was examined for the study of the permanent electric dipole moments of molecular states. A TPR-FWM process of the type omega(4) = omega(1) -omega(2) + omega(3) in a three-state dipolar system was considered. The extraction of data for the difference in permanent dipole moments (Ap) of states involved in TPR was analysed in the case of resonance TPR-FWM, Resonance TPR-FWM measurements were performed in a solution of the polydiacetylene poly-4BCMU. (C) 1998 John Wiley & Sons, Ltd.
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页码：283 / 290
页数：8
相关论文
共 47 条
[11]  
DESCE MB, 1995, CHEM PHYS LETT, V243, P526
[12]   IMPORTANCE OF INITIAL AND FINAL-STATES AS INTERMEDIATE STATES IN 2-PHOTON SPECTROSCOPY OF POLAR-MOLECULES [J].
DICK, B ;
HOHLNEICHER, G .
JOURNAL OF CHEMICAL PHYSICS, 1982, 76 (12) :5755-5760
[13]  
DICK B, 1987, NONLINEAR OPTICAL PR, V2, P162
[14]   ELECTRIC FIELD-INDUCED SPECTRA [J].
DOWS, DA ;
BUCKINGHAM, AD .
JOURNAL OF MOLECULAR SPECTROSCOPY, 1964, 12 (02) :189-&
[15]   2-PHOTON RESONANCE 4-WAVE-MIXING SPECTROSCOPY IN POLAR MEDIA [J].
HADJICHRISTOV, GB ;
STAMOVA, MD ;
KIRCHEVA, PP .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1995, 28 (15) :3441-3451
[16]   ELECTRIC-FIELD EFFECTS ON ORIENTED MOLECULES AND MOLECULAR-CRYSTALS [J].
HOCHSTRASSER, RM .
ACCOUNTS OF CHEMICAL RESEARCH, 1973, 6 (08) :263-269
[17]   THEORETICAL DESCRIPTION OF 2-PHOTON PHASE-CONJUGATION IN POLAR-MOLECULES [J].
HOERNER, C ;
LAVOINE, JP ;
VILLAEYS, AA .
PHYSICAL REVIEW A, 1993, 48 (02) :1564-1572
[18]   RESONANCE ENHANCED COHERENT ANTI-STOKES RAMAN-SCATTERING [J].
HUDSON, B ;
HETHERINGTON, W ;
CRAMER, S ;
CHABAY, I ;
KLAUMINZER, GK .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 1976, 73 (11) :3798-3802
[19]   On the competition between permanent dipole and virtual state two-photon excitation mechanisms, and two-photon optical excitation pathways, in molecular excitation [J].
Jagatap, BN ;
Meath, WJ .
CHEMICAL PHYSICS LETTERS, 1996, 258 (1-2) :293-300
[20]   KRAMERS-KRONIG RELATIONS IN FWM SPECTROSCOPY [J].
KIRCHEVA, PP ;
HADJICHRISTOV, GB .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1994, 27 (16) :3781-3793
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