Shape-controlled synthesis of porous AuPt nanoparticles and their superior electrocatalytic activity for oxygen reduction reaction

被引:24
作者
Sun, Litai [1 ,2 ]
Wang, Hongjing [3 ]
Eid, Kamel [1 ,2 ]
Wang, Liang [1 ,3 ]
机构
[1] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Jilin, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100039, Peoples R China
[3] Zhejiang Univ Technol, Coll Chem Engn, Hangzhou 310014, Zhejiang, Peoples R China
基金
中国国家自然科学基金;
关键词
One-step synthesis; metallic nanoparticles; porous structure; catalyst; oxygen reduction reaction; TUNABLE PORE SIZES; PLATINUM NANOPARTICLES; FUEL-CELLS; FACILE SYNTHESIS; PD; OXIDATION; METHANOL; PERFORMANCE; CATALYSTS; NANODENDRITES;
D O I
10.1080/14686996.2016.1140307
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Control of structure and morphology of Pt-based nanomaterials is of great importance for electrochemical energy conversions. In this work, we report an efficient one-step synthesis of bimetallic porous AuPt nanoparticles (PAuPt NPs) in an aqueous solution. The proposed synthesis is performed by a simple stirring treatment of an aqueous reactive mixture including K2PtCl4, HAuCl4, Pluronic F127 and ascorbic acid at a pH value of 1 without organic solvent or high temperature. Due to their porous structure and bimetallic composition, as-made PAuPt NPs exhibit excellent electrocatalytic activity for oxygen reduction reaction.
引用
收藏
页码:58 / 62
页数:5
相关论文
共 50 条
  • [31] Porous Calcium Manganese Oxide: Preparation and Electrocatalytic Activity of Oxygen Reduction Reaction
    Cao Zhao-Xia
    Ding Yan-Min
    Wang Zhi-Chao
    Mao Xin-Xin
    Yin Yan-Hong
    Yang Shu-Ting
    JOURNAL OF INORGANIC MATERIALS, 2017, 32 (05) : 535 - 542
  • [32] Synthesis of poly(N-vinyl-2-pyrrolidone) adsorbed-AuPt/C bimetallic nanoparticles and their unusual electrocatalytic activity towards methanol tolerant oxygen reduction reaction
    Boopathi, Sidhureddy
    Raju, Chikkili Venkateswara
    Jeyabharathi, Chinnaiah
    Kumar, Shanmugam Senthil
    JOURNAL OF SOLID STATE ELECTROCHEMISTRY, 2016, 20 (02) : 579 - 587
  • [33] Shape-controlled synthesis of Pt nanostructures and evaluation of catalytic and electrocatalytic performance
    Ghosh, Sourov
    Raj, C. Retna
    CATALYSIS SCIENCE & TECHNOLOGY, 2013, 3 (04) : 1078 - 1085
  • [34] Electrocatalytic Activity of Organically Functionalized Silver Nanoparticles in Oxygen Reduction
    He, Guoqiang
    Song, Yang
    Phebus, Bruce
    Liu, Ke
    Deming, Christopher P.
    Hu, Peiguang
    Chen, Shaowei
    SCIENCE OF ADVANCED MATERIALS, 2013, 5 (11) : 1727 - 1736
  • [35] Electrocatalysis of Oxygen Reduction Reaction on Shape-Controlled Pt and Pd Nanoparticles-Importance of Surface Cleanliness and Reconstruction
    Devivaraprasad, Ruttala
    Nalajala, Naresh
    Bera, Bapi
    Neergat, Manoj
    FRONTIERS IN CHEMISTRY, 2019, 7
  • [36] Monodisperse Au-Pd bimetallic alloyed nanoparticles supported on reduced graphene oxide with enhanced electrocatalytic activity towards oxygen reduction reaction
    Lv, Jing-Jing
    Li, Shan-Shan
    Wang, Ai-Jun
    Mei, Li-Ping
    Chen, Jian-Rong
    Feng, Jiu-Ju
    ELECTROCHIMICA ACTA, 2014, 136 : 521 - 528
  • [37] Activity-composition correlation of AuPt alloy nanoparticle catalysts in electrocatalytic reduction of oxygen
    Luo, J
    Njoki, PN
    Lin, Y
    Wang, LY
    Zhong, CJ
    ELECTROCHEMISTRY COMMUNICATIONS, 2006, 8 (04) : 581 - 587
  • [38] Kinetically Controlled Synthesis of PdNi Bimetallic Porous Nanostructures with Enhanced Electrocatalytic Activity
    Zhu, Chengzhou
    Wen, Dan
    Oschatz, Martin
    Holzschuh, Matthias
    Liu, Wei
    Herrmann, Anne-Kristin
    Simon, Frank
    Kaskel, Stefan
    Eychmueller, Alexander
    SMALL, 2015, 11 (12) : 1430 - 1434
  • [39] Synthesis of phosphorus-iridium nanocrystals and their superior electrocatalytic activity for oxygen evolution reaction
    Yin, Lisi
    Yang, Tao
    Ding, Xinran
    He, Maoshuai
    Wei, Wenxian
    Yu, Tingting
    Zhao, Hong
    ELECTROCHEMISTRY COMMUNICATIONS, 2018, 94 : 59 - 63
  • [40] Monodisperse ordered indium-palladium nanoparticles: synthesis and role of indium for boosting superior electrocatalytic activity for ethanol oxidation reaction
    Chen, Yu-Ju
    Chen, Yi-Rui
    Chiang, Cheng-Hsuan
    Tung, Kuo-Lun
    Yeh, Tsung-Kuang
    Tuan, Hsing-Yu
    NANOSCALE, 2019, 11 (07) : 3336 - 3343