Heavy metal and persistent organic compound contamination in soil from Wenling: An emerging e-waste recycling city in Taizhou area, China

被引:277
作者
Tang, Xianjin [1 ]
Shen, Chaofeng [1 ]
Shi, Dezhi [1 ]
Cheema, Sardar A. [1 ]
Khan, Muhammad I. [1 ]
Zhang, Congkai [1 ]
Chen, Yingxu [1 ]
机构
[1] Zhejiang Univ, Inst Environm Sci & Technol, Minist Agr, Key Lab Nonpoint Source Pollut Control, Hangzhou 310029, Zhejiang, Peoples R China
关键词
E-waste; Soil; Heavy metals; PAHs; PCBs; POLYCYCLIC AROMATIC-HYDROCARBONS; POLYCHLORINATED-BIPHENYLS; DISASSEMBLY SITES; FOREST SOILS; PAH SOURCE; PCBS; SAMPLES; DISTRIBUTIONS; INCINERATION; SEDIMENTS;
D O I
10.1016/j.jhazmat.2009.08.134
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The present study was conducted to investigate the levels and sources of heavy metals (Cu, Cr, Cd, Pb, Zn, Hg and As) and persistent organic compounds including polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs) in soils taken from Wenling, an emerging e-waste recycling city in Taizhou, China. The results suggested that most heavy metals exceeded the respective Grade II value of soil quality standards from State Environmental Protection Administration of China and also exceeded the Dutch Optimum values. Total PAHs in soil ranged from 371.8 to 1231.2 mu g/kg, and relatively higher PAHs concentrations were found in soils taken from simple household workshops. PCBs were detectable in ail samples with total concentrations ranging from 52.0 to 5789.5 mu g/kg, which were 2.1-232.5 times higher than that from the reference site (24.9 mu g/kg). Results of this study suggested soil in the Wenling e-waste recycling area were heavily contaminated by heavy metals, PAHs and PCBs. Furthermore, compared with large-scale plants, simple household workshops contributed more heavy metals, PAHs and PCBs pollution to the soil environment, indicating that soil contamination from e-waste recycling in simple household workshops should be given more attention. (C) 2009 Elsevier B.V. All rights reserved.
引用
收藏
页码:653 / 660
页数:8
相关论文
共 48 条
[1]   Polycyclic aromatic hydrocarbons in Norwegian forest soils: Impact of long range atmospheric transport [J].
Aamot, E ;
Steinnes, E ;
Schmid, R .
ENVIRONMENTAL POLLUTION, 1996, 92 (03) :275-280
[2]  
[Anonymous], CHINA ENV SCI
[3]  
*ANZECC NHMRC, 1992, ANZECC B ENV INV LEV
[4]   ORGANIC MICROPOLLUTANTS IN SWISS AGRICULTURE - DISTRIBUTION OF POLYNUCLEAR AROMATIC-HYDROCARBONS (PAH) AND POLYCHLORINATED-BIPHENYLS (PCB) IN SOIL, LIQUID MANURE, SEWAGE-SLUDGE AND COMPOST SAMPLES A COMPARATIVE-STUDY [J].
BERSET, JD ;
HOLZER, R .
INTERNATIONAL JOURNAL OF ENVIRONMENTAL ANALYTICAL CHEMISTRY, 1995, 59 (2-4) :145-165
[5]   Movement and retention of polychlorinated biphenyls in a paddy field of WenTai area in China [J].
Bi, XH ;
Chu, SG ;
Meng, QY ;
Xu, XB .
AGRICULTURE ECOSYSTEMS & ENVIRONMENT, 2002, 89 (03) :241-252
[6]   ECOLOGICAL ASSESSMENT OF A REGION WITH PCB EMISSIONS USING SAMPLES OF SOIL, VEGETATION AND BREAST-MILK - A CASE-STUDY [J].
BOBOVNIKOVA, T ;
DIBTSEVA, A ;
MITROSHKOV, A ;
PLESKACHEVSKAYA, G .
SCIENCE OF THE TOTAL ENVIRONMENT, 1993, 140 :357-364
[7]   Evaluation of sediment contamination by polycyclic aromatic hydrocarbons in the Gironde estuary [J].
Budzinski, H ;
Jones, I ;
Bellocq, J ;
Pierard, C ;
Garrigues, P .
MARINE CHEMISTRY, 1997, 58 (1-2) :85-97
[8]  
CCME, 2003, CAN ENV QUAL GUID SU
[9]   Distributions of polycyclic aromatic hydrocarbons in surface waters, sediments and soils of Hangzhou City, China [J].
Chen, BL ;
Xuan, XD ;
Zhu, LZ ;
Wang, J ;
Gao, YZ ;
Yang, K ;
Shen, XY ;
Lou, BF .
WATER RESEARCH, 2004, 38 (16) :3558-3568
[10]   Contents and sources of polycyclic aromatic hydrocarbons and organochlorine pesticides in vegetable soils of Guangzhou, China [J].
Chen, LG ;
Ran, Y ;
Xing, BS ;
Mai, BX ;
He, JH ;
Wei, XG ;
Fu, JM ;
Sheng, GY .
CHEMOSPHERE, 2005, 60 (07) :879-890