共 65 条
Tailoring the Polymer-Derived Carbon Encapsulated Silicon Nanoparticles for High-Performance Lithium-Ion Battery Anodes
被引:50
作者:

Ma, Qiang
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Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China

Xie, Hongwei
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Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China

Qu, Jiakang
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Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China

Zhao, Zhuqing
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Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China

Zhang, Beilei
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Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China

Song, Qiushi
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Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China

Xing, Pengfei
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Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China

Yin, Huayi
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h-index: 0
机构:
Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China
Northeastern Univ, Minist Educ, Key Lab Data Analyt & Optimizat Smart Ind, Shenyang 110819, Peoples R China Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China
机构:
[1] Northeastern Univ, Sch Met, Shenyang 110819, Peoples R China
[2] Northeastern Univ, Minist Educ, Key Lab Data Analyt & Optimizat Smart Ind, Shenyang 110819, Peoples R China
关键词:
Si@polymer;
Si@C;
anode;
lithium-ion battery;
melamine resin;
carbonization;
SI-C NANOCOMPOSITES;
POROUS SILICON;
AT-CARBON;
HIGH-CAPACITY;
DOPED GRAPHENE;
ACTIVE-SITES;
COMPOSITE;
NITROGEN;
HETEROSTRUCTURES;
ELECTRODES;
D O I:
10.1021/acsaem.9b01463
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
The structure, dopants, and surface area of carbon determine the performance of the core-shell structured silicon and carbon composite (Si@C) anode for Li-ion batteries (LIBs). Herein, we report the synthesis of Si@C composite from poly(vinyl alcohol) (PVA)/melamine resin (MR) dual layer polymer derived carbon encapsulated Si nanoparticles using a polymerization-carbonization approach. The dual polymer layer derived carbon coating has adequate void spaces and dopants, possesses a disordered structure, and seals the Si core sufficiently. Hence, the obtained Si@C-MR anode delivers a superior specific capacity of 1279.3 mA h/g at a current density of 2 A/g and with a retention rate of 88.9% after 500 cycles. A full cell with a Li(Ni0.6Co0.2Mn0.2)O-2 cathode and a prelithiated Si@C-MR anode exhibits a high energy density above 518 Wh/kg and capacity retention of 90.1% after 100 cycles. In parallel, the other three polymer-derived Si@C composites were prepared to study the effect of carbon on the performance of the composite anodes. Overall, constructing a dual-polymer layer holds the promise for rationally designing Si@C anodes for high-performance LIBs through the polymerization-carbonization approach.
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页码:268 / 278
页数:21
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Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA

Cui, Yi
论文数: 0 引用数: 0
h-index: 0
机构:
Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA
SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA
[30]
Electrochemical characterizations on Si and C-coated Si particle electrodes for lithium-ion batteries
[J].
Liu, WR
;
Wang, JH
;
Wu, HC
;
Shieh, DT
;
Yang, MH
;
Wu, NL
.
JOURNAL OF THE ELECTROCHEMICAL SOCIETY,
2005, 152 (09)
:A1719-A1725

Liu, WR
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机构:
Natl Taiwan Univ, Dept Chem Engn, Taipei 106, Taiwan Natl Taiwan Univ, Dept Chem Engn, Taipei 106, Taiwan

Wang, JH
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机构: Natl Taiwan Univ, Dept Chem Engn, Taipei 106, Taiwan

Wu, HC
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h-index: 0
机构: Natl Taiwan Univ, Dept Chem Engn, Taipei 106, Taiwan

Shieh, DT
论文数: 0 引用数: 0
h-index: 0
机构: Natl Taiwan Univ, Dept Chem Engn, Taipei 106, Taiwan

Yang, MH
论文数: 0 引用数: 0
h-index: 0
机构: Natl Taiwan Univ, Dept Chem Engn, Taipei 106, Taiwan

Wu, NL
论文数: 0 引用数: 0
h-index: 0
机构: Natl Taiwan Univ, Dept Chem Engn, Taipei 106, Taiwan