Temperature Dependence of the Nitrogen-Vacancy Magnetic Resonance in Diamond

被引：538
作者：
Acosta, V. M. [1 ]
Bauch, E. [1 ,2 ]
Ledbetter, M. P. [1 ]
Waxman, A. [3 ]
Bouchard, L-S. [4 ]
Budker, D. [1 ,5 ]
机构：
[1] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
[2] Tech Univ Berlin, D-10623 Berlin, Germany
[3] Ben Gurion Univ Negev, Dept Phys, IL-84105 Beer Sheva, Israel
[4] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA
[5] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA
来源：
PHYSICAL REVIEW LETTERS | 2010年 / 104卷 / 07期
基金：
美国国家科学基金会;
关键词：
ATOMIC MAGNETOMETER; DEFECT CENTERS; SPIN; MICROSCOPY; NMR;
D O I：
10.1103/PhysRevLett.104.070801
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
The temperature dependence of the magnetic-resonance spectra of nitrogen-vacancy (NV(-)) ensembles in the range of 280-330 K was studied. Four samples prepared under different conditions were analyzed with NV(-) concentrations ranging from 10 ppb to 15 ppm. For all samples, the axial zero-field splitting (ZFS) parameter D was found to vary significantly with temperature, T, as dD/dT = -74.2(7) kHz/K. The transverse ZFS parameter E was nonzero (between 4 and 11 MHz) in all samples, and exhibited a temperature dependence of dE/(EdT) = -1.4(3) x 10(-4) K(-1). The results might be accounted for by considering local thermal expansion. The temperature dependence of the ZFS parameters presents a significant challenge for diamond magnetometers and may ultimately limit their bandwidth and sensitivity.
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页数：4
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