Simulation of time-dependent resonant inelastic x-ray scattering using nonequilibrium dynamical mean-field theory

被引:12
|
作者
Eckstein, Martin [1 ]
Werner, Philipp [2 ]
机构
[1] Univ Erlangen Nurnberg, Dept Phys, D-91058 Erlangen, Germany
[2] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland
基金
欧洲研究理事会;
关键词
SPECTROSCOPY; ENERGY;
D O I
10.1103/PhysRevB.103.115136
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We develop a framework to evaluate the time-dependent resonant inelastic x-ray scattering (RIXS) signal with the use of nonequilibrium dynamical mean-field theory simulations. The approach is based on the solution of a time-dependent impurity model which explicitly incorporates the probe pulse. It avoids the need to compute four-point correlation functions and can in principle be combined with different impurity solvers. This opens a path to study time-resolved RIXS processes in multiorbital systems. The approach is exemplified with a study of the RIXS signal of a melting Mott antiferromagnet.
引用
收藏
页数:11
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