Spatially heterogeneous dynamics in liquids: insights from simulation

被引：377

作者：

Glotzer, SC

机构：

[1] NIST, Div Polymers, Gaithersburg, MD 20899 USA

[2] NIST, Ctr Theoret & Computat Mat Sci, Gaithersburg, MD 20899 USA

来源：

JOURNAL OF NON-CRYSTALLINE SOLIDS | 2000年 / 274卷 / 1-3期

关键词：

D O I：

10.1016/S0022-3093(00)00225-8

中图分类号：

TQ174 [陶瓷工业]; TB3 [工程材料学];

学科分类号：

0805 ; 080502 ;

摘要：

In this paper, review of recent theoretical and simulation work on dynamical heterogeneity and correlated particle motion in glass-forming liquids and polymers is presented. Evidence for increasing mobility fluctuations in these systems with decreasing temperature, and the relationship between dynamical heterogeneity and decoupling of diffusion and structural relaxation is described. The relationship between dynamical heterogeneity, string-like collective motion, the clustering of strings, and mode-coupling theory is briefly discussed. (C) 2000 Elsevier Science B.V. All rights reserved.

引用

页码：342 / 355

页数：14

共 50 条

[21] Dynamics of an EIS spatially heterogeneous rabies model
Hu, Yaru
Wang, Jinfeng
[J]. JOURNAL OF DIFFERENTIAL EQUATIONS, 2024, 384 : 326 - 351
[22] Classical Molecular Dynamics Simulation of Glyonic Liquids: Structural Insights and Relation to Conductive Properties
Hei, Bai
Pemberton, Jeanne E.
Schwartz, Steven D.
[J]. JOURNAL OF PHYSICAL CHEMISTRY B, 2023, 127 (04) : 921 - 931
[23] Spatially heterogeneous dynamics and locally arrested density fluctuations from first principles
Lira-Escobedo, J.
Velez-Cordero, J. R.
Ramirez-Gonzalez, Pedro E.
[J]. PHYSICS OF FLUIDS, 2022, 34 (03)
[24] The partition and transport behavior of cytotoxic ionic liquids (ILs) through the DPPC bilayer: Insights from molecular dynamics simulation
Koli, Mokhtar Ganjali
Azizi, Khaled
[J]. MOLECULAR MEMBRANE BIOLOGY, 2016, 33 (3-5) : 64 - 75
[25] Heterogeneous dynamics in liquids: fluctuations in space and time
Richert, R
[J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 2002, 14 (23) : R703 - R738
[26] Effects of lowering temperature and raising pressure on the spatially heterogeneous dynamics of glass-forming van der Waals liquids
Grzybowski, A.
Kolodziejczyk, K.
Koperwas, K.
Grzybowska, K.
Paluch, M.
[J]. PHYSICAL REVIEW B, 2012, 85 (22):
[27] Comparison of Heterogeneous Dynamics in Ionic Liquids and Ionically Conducting Glasses from Molecular Dynamics Simulations
Habasaki, Junko
Ngai, K. L.
[J]. JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2010, 79
[28] Insights into polyunsaturated lipids from molecular dynamics simulation
Feller, S
[J]. BIOPHYSICAL JOURNAL, 2004, 86 (01) : 366A - 366A
[29] Synchrony, extinction, and dynamics of spatially segregated, heterogeneous populations
Matter, SF
[J]. ECOLOGICAL MODELLING, 2001, 141 (1-3) : 217 - 226
[30] DYNAMICS OF SPATIALLY HETEROGENEOUS VIRAL MODEL WITH TIME DELAY
Yang, Hong
Wei, Junjie
[J]. COMMUNICATIONS ON PURE AND APPLIED ANALYSIS, 2020, 19 (01) : 85 - 102

← 1 2 3 4 5 →