Residential Tap Water Contamination Following the Freedom Industries Chemical Spill: Perceptions, Water Quality, and Health Impacts

被引:116
作者
Whelton, Andrew J. [1 ,2 ]
McMillan, LaKia [3 ]
Connell, Matt [3 ]
Kelley, Keven M. [3 ]
Gill, Jeff P. [3 ]
White, Kevin D. [3 ]
Gupta, Rahul [4 ]
Dey, Rajarshi [5 ]
Novy, Caroline [3 ]
机构
[1] Purdue Univ, Div Environm & Ecol Engn, W Lafayette, IN 47907 USA
[2] Purdue Univ, Lyles Sch Civil Engn, W Lafayette, IN 47907 USA
[3] Univ S Alabama, Dept Civil Engn, Mobile, AL 36688 USA
[4] Kanawha Charleston Hlth Dept, Charleston, WV 25301 USA
[5] Univ S Alabama, Dept Math & Stat, Mobile, AL 36688 USA
基金
美国国家科学基金会;
关键词
Water quality - Water supply - Disease control - Surveys - Sewage - Polyethylenes - Water pollution - Crosslinking - Hazardous materials spills;
D O I
10.1021/es5040969
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
During January 2014, an industrial solvent contaminated West Virginias Elk River and 15% of the state populations tap water. A rapid in-home survey and water testing was conducted 2 weeks following the spill to understand resident perceptions, tap water chemical levels, and premise plumbing flushing effectiveness. Water odors were detected in all 10 homes sampled before and after premise plumbing flushing. Survey and medical data indicated flushing caused adverse health impacts. Bench-scale experiments and physiochemical property predictions showed flushing promoted chemical volatilization, and contaminants did not appreciably sorb into cross-linked polyethylene (PEX) pipe. Flushing reduced tap water 4-methylcyclohexanemethanol (4-MCHM) concentrations within some but not all homes. 4-MCHM was detected at unflushed (<10 to 420 mu g/L) and flushed plumbing systems (<10 to 96 mu g/L) and sometimes concentrations differed among faucets within each home. All waters contained less 4-MCHM than the 1000 mu g/L Centers for Disease Control drinking water limit, but one home exceeded the 120 mu g/L drinking water limit established by independent toxicologists. Nearly all households refused to resume water use activities after flushing because of water safety concerns. Science based flushing protocols should be developed to expedite recovery, minimize health impacts, and reduce concentrations in homes when future events occur.
引用
收藏
页码:813 / 823
页数:11
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