Advanced Pd-based nanomaterials for electro-catalytic oxygen reduction in fuel cells: A review

被引：62
作者：
Sanij, Fereshteh Dehghani [1 ]
Balakrishnan, Prabhuraj [1 ]
Leung, Puiki [2 ]
Shah, Akeel [3 ]
Su, Huaneng [1 ]
Xu, Qian [1 ]
机构：
[1] Jiangsu Univ, Inst Energy Res, Zhenjiang 212013, Jiangsu, Peoples R China
[2] Univ Southampton, Fac Engn & Environm, Southampton SO17 1BJ, Hants, England
[3] Chongqing Univ, MOE Key Lab Low Grade Energy Utilizat Technol & S, Chongqing 400030, Peoples R China
来源：
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2021年 / 46卷 / 27期
基金：
中国博士后科学基金; 中国国家自然科学基金;
关键词：
Oxygen reduction reaction; Pd-based nanocatalyst; Cathode; PEMFC; DMFC; AEMFC; CARBON-SUPPORTED PD; REDUCED GRAPHENE OXIDE; PALLADIUM NANOPARTICLES; ELECTROCATALYTIC ACTIVITY; CATHODE CATALYSTS; RECENT PROGRESS; ELECTROCHEMICAL REDUCTION; ALLOYED NANOPARTICLES; NANOCHAIN NETWORKS; FACILE SYNTHESIS;
D O I：
10.1016/j.ijhydene.2021.01.185
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Devising cost-effective and high-performance nanocatalysts for the inherently slow oxygen reduction reaction (ORR) represents a critical hurdle in the commercial improvement of fuel cells for energy conversion. Recently, considerable attempts have concentrated on exploring Pd-based nanocatalysts with advanced stability to utilize as substitutes for Pt. In this review, we first describe ORR mechanisms and summarize research conducted with Pd electro-catalysts, including single and alloyed Pd nanostructures on different substrates. The application of Pd catalysts as cathode nanomaterials in proton exchange membrane fuel cells (PEMFCs), direct methanol fuel cells (DMFCs), and anion exchange membrane fuel cells (AEMFCs) is also reviewed. The insights into the connections between catalytic performance, structure, and preparation process are addressed. In particular, approaches for fabricating efficient Pd electro-catalysts, such as increasing the number of reactive centers and modifying nanoparticle-support interactions, are discussed. Challenges and prospects for upcoming investigations in developing desirable ORR nanocatalysts are highlighted. (c) 2021 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码：14596 / 14627
页数：32
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