Saturated near-resonant refractive optical nonlinearity in CdTe quantum dots

被引:26
作者
Dancus, I. [1 ]
Vlad, V. I. [1 ]
Petris, A. [1 ]
Gaponik, N. [2 ]
Lesnyak, V. [2 ]
Eychmueller, A. [2 ]
机构
[1] Natl Inst Lasers Plasma & Radiat Phys, Laser Dept, Bucharest 077125, Romania
[2] Tech Univ Dresden, D-01062 Dresden, Germany
关键词
NANOCRYSTALS;
D O I
10.1364/OL.35.001079
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
In this work, we report on an experimental investigation of the nonlinear optical properties near the first electronic resonance of thiol-capped CdTe quantum dots (QDs) being in the strong confinement regime. Using a cw laser excitation in a Z-scan experimental setup, we show the presence of saturated Kerr-type nonlinear optical properties of the QDs, at low intensity levels. The large optical nonlinearity and the control of the linear and nonlinear optical properties by the size of the QDs are of special interest for applications in integrated nanophotonic devices. (C) 2010 Optical Society of America
引用
收藏
页码:1079 / 1081
页数:3
相关论文
共 12 条
[1]   BELOW-BAND-GAP 3RD-ORDER OPTICAL NONLINEARITY OF NANOMETER-SIZE SEMICONDUCTOR CRYSTALLITES [J].
COTTER, D ;
BURT, MG ;
MANNING, RJ .
PHYSICAL REVIEW LETTERS, 1992, 68 (08) :1200-1203
[2]  
Dancus I, 2008, J OPTOELECTRON ADV M, V10, P149
[3]   NONLINEAR-OPTICAL PROPERTIES OF SEMICONDUCTOR QUANTUM DOTS AND THEIR CORRELATION WITH THE PRECIPITATION STAGE [J].
GAPONENKO, SV ;
WOGGON, U ;
SALEH, M ;
LANGBEIN, W ;
UHRIG, A ;
MULLER, M ;
KLINGSHIRN, C .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1993, 10 (10) :1947-1954
[4]   Non-linear optical measurements and crystalline characterization of CdTe nanoparticles produced by the 'electropulse' technique [J].
Loicq, J ;
Renotte, Y ;
Delplancke, JL ;
Lion, Y .
NEW JOURNAL OF PHYSICS, 2004, 6
[5]   The second hyperpolarizability of CdTe nanocrystals using polarization-re solved degenerate four-wave mixing [J].
Ma, S. M. ;
Seo, J. T. ;
Yang, Q. ;
Battle, R. ;
Creekmore, L. ;
Lee, K. ;
Tabibi, B. ;
Yu, W. .
APPLIED SURFACE SCIENCE, 2007, 253 (15) :6612-6615
[6]   Nonlinear optical properties of thiol-capped CdTe quantum dots in nonresonant region [J].
Pan, Lingyun ;
Tamai, Naoto ;
Kamada, Kenji ;
Deki, Shigehito .
APPLIED PHYSICS LETTERS, 2007, 91 (05)
[7]   Time- and spectrally-resolved four-wave mixing in single CdTe/ZnTe quantum dots [J].
Patton, B. ;
Langbein, W. ;
Woggon, U. ;
Maingault, L. ;
Mariette, H. .
PHYSICAL REVIEW B, 2006, 73 (23)
[8]   SYNTHESIS AND CHARACTERIZATION OF SURFACE-MODIFIED COLLOIDAL CDTE QUANTUM DOTS [J].
RAJH, T ;
MICIC, OI ;
NOZIK, AJ .
JOURNAL OF PHYSICAL CHEMISTRY, 1993, 97 (46) :11999-12003
[9]   Aqueous synthesis of thiol-capped CdTe nanocrystals:: State-of-the-art [J].
Rogach, Andrey L. ;
Franzl, Thomas ;
Klar, Thomas A. ;
Feldmann, Jochen ;
Gaponik, Nikolai ;
Lesnyak, Vladimir ;
Shavel, Alexey ;
Eychmueller, Alexander ;
Rakovich, Yuri P. ;
Donegan, John F. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2007, 111 (40) :14628-14637
[10]   Cadmium chalcogenide semiconductor nanocrystals for optical power limiting application [J].
Seo, JT ;
Ma, S ;
Lee, K ;
Tabibi, B ;
Rankins, C ;
Muhoro, P ;
Mangana, J ;
Pompey, C ;
Creekmore, S ;
Xie, Z ;
Peng, X ;
Qu, J ;
Yu, W ;
Wang, A ;
Jung, S ;
Ruh, H .
11TH INTERNATIONAL CONFERENCE ON II-VI COMPOUNDS (II-VI 2003), PROCEEDINGS, 2004, 1 (04) :771-774