The South Asian monsoon-pollution pump and purifier

被引:111
作者
Lelieveld, J. [1 ,2 ]
Bourtsoukidis, E. [1 ]
Bruehl, C. [1 ]
Fischer, H. [1 ]
Fuchs, H. [3 ]
Harder, H. [1 ]
Hofzumahaus, A. [3 ]
Holland, F. [3 ]
Marno, D. [1 ]
Neumaier, M. [4 ]
Pozzer, A. [1 ]
Schlager, H. [5 ]
Williams, J. [1 ,2 ]
Zahn, A. [4 ]
Ziereis, H. [5 ]
机构
[1] Max Planck Inst Chem, D-55128 Mainz, Germany
[2] Cyprus Inst, CY-1645 Nicosia, Cyprus
[3] Res Ctr Julich, Inst Energy & Climate Res, D-52425 Julich, Germany
[4] Karlsruhe Inst Technol, D-76021 Karlsruhe, Germany
[5] Germany Aerosp Ctr, Inst Atmospher Phys, D-82234 Oberpfaffenhofen, Germany
关键词
INDIAN-OCEAN EXPERIMENT; IN-SITU MEASUREMENTS; TRACE GASES; STRATOSPHERE; ANTICYCLONE; CHEMISTRY; TRANSPORT; CLIMATE; AEROSOLS; IMPACTS;
D O I
10.1126/science.aar2501
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Air pollution is growing fastest in monsoon-affected South Asia. During the drywintermonsoon, the fumes disperse toward the Indian Ocean, creating a vast pollution haze, but their fate during the wet summer monsoon has been unclear. We performed atmospheric chemistry measurements by aircraft in the Oxidation Mechanism Observations campaign, sampling the summer monsoon outflow in the upper troposphere between the Mediterranean and the Indian Ocean. The measurements, supported by model calculations, show that the monsoon sustains a remarkably efficient cleansing mechanism by which contaminants are rapidly oxidized and deposited to Earth's surface. However, some pollutants are lofted above the monsoon clouds and chemically processed in a reactive reservoir before being redistributed globally, including to the stratosphere.
引用
收藏
页码:270 / +
页数:4
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