Tensor Network Simulation of Non-Markovian Dynamics in Organic Polaritons

被引：96

作者：

del Pino, Javier ^{[1
,2
]}

Schroder, Florian A. Y. N. ^{[3
]}

Chin, Alex W. ^{[3
,4
]}

Feist, Johannes ^{[1
,2
]}

Garcia-Vidal, Francisco J. ^{[1
,2
,5
]}

机构：

[1] Univ Autonoma Madrid, Dept Fis Teor Mat Condensada, E-28049 Madrid, Spain

[2] Univ Autonoma Madrid, Condensed Matter Phys Ctr IFIMAC, E-28049 Madrid, Spain

[3] Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England

[4] Sorbonne Univ, Inst NanoSci Paris, 4 Pl Jussieu,Boite Courrier 840, F-75252 Paris 05, France

[5] DIPC, E-20018 Donostia San Sebastian, Spain

来源：

PHYSICAL REVIEW LETTERS | 2018年 / 121卷 / 22期

基金：

欧洲研究理事会; 英国工程与自然科学研究理事会;

关键词：

MATRIX RENORMALIZATION-GROUP; ROOM-TEMPERATURE; MOLECULES; CAVITIES;

D O I：

10.1103/PhysRevLett.121.227401

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We calculate the exact many-body time dynamics of polaritonic states supported by an optical cavity filled with organic molecules. Optical, vibrational, and radiative processes are treated on an equal footing employing the time-dependent variational matrix product states algorithm. We demonstrate signatures of non-Markovian vibronic dynamics and its fingerprints in the far-field photon emission spectrum at arbitrary light-matter interaction scales, ranging from the weak to the strong coupling regimes. We analyze both the single-and many-molecule cases, showing the crucial role played by the collective motion of molecular nuclei and dark states in determining the polariton dynamics and the subsequent photon emission.

引用

页数：7

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