Exfoliated and plicated g-C3N4 nanosheets for efficient photocatalytic organic degradation and hydrogen evolution

被引:49
作者
Beyhaqi, Ahmad [1 ]
Azimi, Seyed Mohammad Taghi [1 ]
Chen, Zhihong [1 ]
Hu, Chun [1 ]
Zeng, Qingyi [1 ,2 ]
机构
[1] Guangzhou Univ, Inst Environm Res Greater Bay, Guangzhou 510006, Peoples R China
[2] Univ South China, Sch Resources & Environm & Safety Engn, Hengyang 421001, Hunan, Peoples R China
基金
中国国家自然科学基金; 国家重点研发计划;
关键词
G-C3N4; nanosheets; Acidic etching; Photocatalysis; GRAPHITIC CARBON NITRIDE; STRUCTURAL DISTORTION; CHARGE SEPARATION; ENHANCEMENT; REDUCTION;
D O I
10.1016/j.ijhydene.2021.03.174
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Exfoliated and plicated g-C3N4 nanosheets (CNsF) were prepared through a thermalchemical exfoliation in which the bulk g-C3N4 was obtained first under thermal exfoliation, and then was exposed to an acidic etching using hydrofluoric acid under hydrothermal condition. The acidic etching not only exfoliated g-C3N4 nanosheets by disrupting weak van der Waals forces between layers, which led to formation of a monolayer or a few layers of g-C3N4 nanosheets, but also made disordered defects on its surface and created
引用
收藏
页码:20547 / 20559
页数:13
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