Interaction mechanism of heavy metal ions with the nanostructured zeolites surface-Adsorption, electrokinetic and XPS studies

被引：41
作者：
Medykowska, Magdalena [1 ]
Wisniewska, Malgorzata [1 ]
Szewczuk-Karpisz, Katarzyna [2 ]
Panek, Rafal [3 ]
机构：
[1] Marie Curie Sklodowska Univ, Inst Chem Sci, Fac Chem, Dept Radiochem & Environm Chem, Mar Curie Sklodowska Sq 3, PL-20031 Lublin, Poland
[2] Polish Acad Sci, Inst Agrophys, Doswiadczalna 4, PL-20290 Lublin, Poland
[3] Lublin Univ Technol, Fac Civil Engn & Architecture, Dept Bldg Mat Engn & Geoengn, Nadbystrzycka St 40, PL-20618 Lublin, Poland
来源：
JOURNAL OF MOLECULAR LIQUIDS | 2022年 / 357卷
关键词：
Na-X synthetic zeolite; Na-P1 synthetic zeolite; Zeolite-carbon composite; Fly ash precursor; Pb(II) and Zn(II) removal; XPS study; nanostructured solid; RAY PHOTOELECTRON-SPECTROSCOPY; ZERO-VALENT IRON; AQUEOUS-SOLUTION; SOIL CONTAMINATION; POLYACRYLIC-ACID; FLY-ASH; REMOVAL; PB(II); WATER; PB;
D O I：
10.1016/j.molliq.2022.119144
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The aim of the research was to compare the mechanisms of heavy metal ions (Pb(II) and Zn(II)) adsorption on the surfaces of nanostructured synthetic zeolites: Na-X, Na-P1, their carbon composites: Na-X (C), Na-P1 (C) and the precursor of these structures - high-carbon fly ash (HC FA). The research was carried out in single and mixed adsorbate systems. Heavy metals were selected on the basis of their toxicity and their occurrence in the natural environment. The adsorption-desorption and electrokinetic data were obtained by means of inductively coupled plasma-optical emission spectrometry, potentiometric titrations and zeta potential determination. Additionally, the X-ray photoelectron spectroscopy (XPS) was applied to specify the elemental composition of the solids surfaces and the chemical forms of adsorbed metals. (c) 2022 The Author(s). Published by Elsevier B.V. This is an open access article under the CC BY-NC license (http://creativecommons.org/licenses/by-nc/4.0/).
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页数：11
相关论文
共 53 条
[1]   Phytoremediation of heavy metals-Concepts and applications [J].
Ali, Hazrat ;
Khan, Ezzat ;
Sajad, Muhammad Anwar .
CHEMOSPHERE, 2013, 91 (07) :869-881
[2]   Synthesis of zeolite-carbon composites using high-carbon fly ash and their adsorption abilities towards petroleum substances [J].
Bandura, Lidia ;
Panek, Rafal ;
Madej, Jaroslaw ;
Franus, Wojciech .
FUEL, 2021, 283
[3]   Correlation between ionic radius and thermal decomposition of Fe(II), Co(II), Ni(II), Cu(II) and Zn(II) diethanoldithiocarbamates [J].
Breviglieri, ST ;
Cavalheiro, ÉTG ;
Chierice, GO .
THERMOCHIMICA ACTA, 2000, 356 (1-2) :79-84
[4]   X-ray photoelectron spectroscopy and auger electron spectroscopy studies of Al-doped ZnO films [J].
Chen, M ;
Wang, X ;
Yu, YH ;
Pei, ZL ;
Bai, XD ;
Sun, C ;
Huang, RF ;
Wen, LS .
APPLIED SURFACE SCIENCE, 2000, 158 (1-2) :134-140
[5]  
Cheng T, 2018, IRAN J CHEM CHEM ENG, V37, P61
[6]   The effect of temperature on the adsorption and conformation of polyacrylic acid macromolecules at the ZrO2-polymer solution interface [J].
Chibowski, S ;
Wisniewska, M ;
Mazur, EO .
POWDER TECHNOLOGY, 2004, 141 (1-2) :12-19
[7]   Influence of heavy metals on C and N mineralisation and microbial biomass in Zn-, Pb-, Cu-, and Cd-contaminated soils [J].
Dai, J ;
Becquer, T ;
Rouiller, JH ;
Reversat, G ;
Bernhard-Reversat, F ;
Lavelle, P .
APPLIED SOIL ECOLOGY, 2004, 25 (02) :99-109
[8]  
Demidowicz M., 2020, STATE ENV GORZW WIEL, P100
[9]   Copper (II) Removal from Water by Natural Zeolites [J].
Dursun, Sukru ;
Argun, M. Emin ;
Celik, Nazan ;
Celebi, Fatma .
SURVIVAL AND SUSTAINABILITY: ENVIRONMENTAL CONCERNS IN THE 21ST CENTURY, 2011, :831-840
[10]   X-ray photoelectron spectroscopy: Progress and perspectives [J].
Fadley, C. S. .
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2010, 178 :2-32
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