Uranium isotopes in the Balkan's environment and foods following the use of depleted uranium in the war

Immediately after the Balkan's war in 1999, there has been widespread international concern about the environmental contamination with depleted uranium (DU) from ammunitions used in the conflict. Exposure of military staff and local populations to uranium metal and to its ionizing radiation were feared as potential causes for leukemia and other diseases in that region. In January 2001 a scientific mission was carried out by Portugal to evaluate those issues. A large number of environmental and food samples collected in Kosovo and Bosnia-Herzegovina, such as soils, water, aerosols, vegetables, bread, and meat were analyzed by radiochemistry and alpha spectrometry. Results of the analyses for total uranium and individual uranium isotopes are presented. Uranium in agriculture soils in Kosovo and Bosnia-Herzegovina averaged 1.8 +/- 0.8 mg kg(-1) and 3 +/- 1 mg kg(-1), while concentrations in drinking water from public supplies averaged 0.5 +/- 0.2 mu g L(-1) and 0.4 +/- 0.3 mu g L(-1), respectively. Results on soils indicated also that environmental contamination by DU was much localized and confined to the areas of ammunition impact Concentrations of uranium in most of the environmental and food samples were comparable to concentrations of uranium measured in other European regions, such as Portugal and United Kingdom, and uranium isotopic ratios were in general compatible with isotopic ratios typical of natural uranium. However, a few samples displayed modified uranium isotopic ratios and could have been contaminated by DU. Implications of DU in radiation exposure of the population and in environmental contamination are discussed. (C) 2010 Elsevier Ltd. All rights reserved.