High-efficient Synthesis and Photocatalytic Properties of Ag/AgBr/TiO2 Monolithic Photocatalysts Using Sodium Alginate as Substrate

被引:9
作者
Tong Qin [1 ]
Dong Ya-Mei [1 ]
Yan Liang [1 ]
He Dan-Nong [1 ,2 ]
机构
[1] Natl Engn Res Ctr Nanotechnol, Shanghai 200241, Peoples R China
[2] Shanghai Jiao Tong Univ, Sch Mat Sci & Engn, Shanghai 200240, Peoples R China
基金
上海市科技启明星计划;
关键词
sodium alginate; Ag/AgBr/TiO2; photocatlyst; monolithic photocatalysts; visible light; RHODAMINE-B; TIO2; FILMS; FABRICATION; COMPOSITE; CLAY;
D O I
10.15541/jim20160481
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
SA-Ag/AgBr/TiO2 monolithic photocatalysts with uniform particle size distribution was synthesized by using sodium alginate as a substrate. Its structure and morphology were characterized by XRD, XPS, SEM, TEM, and HRTEM. The optical properties and the surface area of the SA-Ag/AgBr/TiO2 monolithic photocatalysts were characterized by FT-IR and BET. The as-prepared photocatalyst with good stability exhibited enhanced photocatalytic performance for degradation of RhB solution under both UV and visible light. The SA-Ag/AgBr/TiO2 monolithic photocatalyst with 12wt% Ag/AgBr/TiO2 display optimum properties i.e. about 100% degradation rate for the RhB solution for 60 min under UV irradiation and 54.1% degradation rate for the RhB solution under visible light irradiation for 120 min. Besides, after 5 cycles, the RhB degradation rate still keeps higher than 96%, showing an excellent reusability of the photocatalysts. The as-prepared SA-Ag/AgBr/TiO2 monolithic photocatalysts may effectively solve the problems including photocatalytic activity, secondary pollution and photocatalyst recycling.
引用
收藏
页码:637 / 642
页数:6
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