Arene Amination Instead of Fluorination: Substitution Pattern Governs the Reactivity of Dialkoxybenzenes with Selectfluor

被引:8
作者
Capilato, Joseph N. [1 ]
Lectka, Thomas [1 ]
机构
[1] Johns Hopkins Univ, Dept Chem, Baltimore, MD 21218 USA
基金
美国国家科学基金会;
关键词
C-H AMINATION; AROMATIC-SUBSTITUTION; CHEMISTRY; LIGANDS; FUNCTIONALIZATION; HETEROCYCLES; MECHANISM; LIQUID; BONDS;
D O I
10.1021/acs.joc.1c00231
中图分类号
O62 [有机化学];
学科分类号
070303 ; 081704 ;
摘要
Arene substitution patterns are well-known to affect the regioselectivity of a given transformation but not necessarily the type of reactivity. Herein, we report that the substitution pattern of alkoxyarenes dictates whether a putative one-electron or two-electron reaction predominates in reactions with Selectfluor. A series of amination products is presented, resulting from the single-electron oxidation of electron-rich arenes followed by direct C-H to C-N bond formation. We demonstrate the ability of this transformation to synthesize medicinally and biologically relevant nitrogen heterocycles. Lastly, this unusual "mechanistic switch" is probed with computational chemistry and competition experiments.
引用
收藏
页码:5771 / 5777
页数:7
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