Enhanced photocatalytic performance of ultrasound treated GO/TiO2 composite for photocatalytic degradation of salicylic acid under sunlight illumination

被引:143
作者
Hunge, Y. M. [1 ]
Yadav, A. A. [1 ]
Dhodamani, A. G. [3 ]
Suzuki, N. [1 ]
Terashima, C. [1 ]
Fujishima, A. [1 ]
Mathe, V. L. [2 ]
机构
[1] Tokyo Univ Sci, Photocatalysis Int Res Ctr, Noda, Chiba 2788510, Japan
[2] Savitribai Phule Pune Univ, Dept Phys, Pune 411007, Maharashtra, India
[3] Shivaji Univ, Dept Chem, Kolhapur 416004, Maharashtra, India
关键词
Hydrothermal method; Photocatalytic degradation; Salicylic acid; Chemical oxygen demand; REDUCED GRAPHENE OXIDE; ASSISTED PHOTOELECTROCATALYTIC DEGRADATION; TIO2; WO3; SHEETS; FILMS;
D O I
10.1016/j.ultsonch.2019.104849
中图分类号
O42 [声学];
学科分类号
070206 ; 082403 ;
摘要
The current research work deals with the preparation of TiO2 and GO/TiO2 composite by simple, chemical, cost effective hydrothermal method. Graphene oxide (GO) is prepared by modified Hummer's method. Dispersion of GO is achieved by an ultrasonic cleaning bath for 1 h. using a power of 200 W and at a frequency of 40 kHz. The prepared catalyst material is characterized by different characterization techniques. XRD study confirms the prepared material is polycrystalline in nature. The synthesized TiO2 and GO/TiO2 photocatalyst materials are used to study the photocatalytic degradation of salicylic acid under sunlight illumination. GO/TiO2 composite shows superior photocatalytic activity than TiO2. GO/TiO2 composite shows 57% degradation of salicylic acid. Mineralization of salicylic acid is studied using chemical oxygen demand.
引用
收藏
页数:6
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共 40 条
[11]   Photoelectrochemical mineralization of textile diazo dye pollutants using nanocrystalline WO3 electrodes [J].
Hepel, M ;
Luo, J .
ELECTROCHIMICA ACTA, 2001, 47 (05) :729-740
[12]   Agent-free synthesis of graphene oxide/transition metal oxide composites and its application for hydrogen storage [J].
Hong, Won G. ;
Kim, Byung Hoon ;
Lee, Sang Moon ;
Yu, Han Young ;
Yun, Yong Ju ;
Jun, Yongseok ;
Lee, Jin Bae ;
Kim, Hae Jin .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2012, 37 (09) :7594-7599
[13]   Photocatalytic hydrogen production using TiO2 nanogranules prepared by hydrothermal route [J].
Hunge, Y. M. ;
Yadav, A. A. ;
Mathe, V. L. .
CHEMICAL PHYSICS LETTERS, 2019, 731
[14]   Sonochemical synthesis of CZTS photocatalyst for photocatalytic degradation of phthalic acid [J].
Hunge, Y. M. ;
Yadav, A. A. ;
Liu, S. ;
Mathe, V. L. .
ULTRASONICS SONOCHEMISTRY, 2019, 56 :284-289
[15]   A multifunctional ZnO thin film based devices for photoelectrocatalytic degradation of terephthalic acid and CO2 gas sensing applications [J].
Hunge, Y. M. ;
Yadav, A. A. ;
Kulkarni, S. B. ;
Mathe, V. L. .
SENSORS AND ACTUATORS B-CHEMICAL, 2018, 274 :1-9
[16]   Ultrasound assisted synthesis of WO3-ZnO nanocomposites for brilliant blue dye degradation [J].
Hunge, Y. M. ;
Yadav, A. A. ;
Mathe, V. L. .
ULTRASONICS SONOCHEMISTRY, 2018, 45 :116-122
[17]   Oxidative degradation of phthalic acid using TiO2 photocatalyst [J].
Hunge, Y. M. ;
Yadav, A. A. ;
Mathe, V. L. .
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2018, 29 (08) :6183-6187
[18]   Photoelectrocatalytic degradation of sugarcane factory wastewater using WO3/ZnO thin films [J].
Hunge, Y. M. ;
Yadav, A. A. ;
Mohite, B. M. ;
Mathe, V. L. ;
Bhosale, C. H. .
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2018, 29 (05) :3808-3816
[19]   Photoelectrocatalytic degradation of oxalic acid using WO3 and stratified WO3/TiO2 photocatalysts under sunlight illumination [J].
Hunge, Y. M. ;
Mahadik, M. A. ;
Moholkar, A. V. ;
Bhosale, C. H. .
ULTRASONICS SONOCHEMISTRY, 2017, 35 :233-242
[20]   Photoelectrocatalytic degradation of methyl red using sprayed WO3 thin films under visible light irradiation [J].
Hunge, Y. M. ;
Mohite, V. S. ;
Kumbhar, S. S. ;
Rajpure, K. Y. ;
Moholkar, A. V. ;
Bhosale, C. H. .
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2015, 26 (11) :8404-8412