Enhanced photocatalytic performance of ultrasound treated GO/TiO2 composite for photocatalytic degradation of salicylic acid under sunlight illumination

被引:142
作者
Hunge, Y. M. [1 ]
Yadav, A. A. [1 ]
Dhodamani, A. G. [3 ]
Suzuki, N. [1 ]
Terashima, C. [1 ]
Fujishima, A. [1 ]
Mathe, V. L. [2 ]
机构
[1] Tokyo Univ Sci, Photocatalysis Int Res Ctr, Noda, Chiba 2788510, Japan
[2] Savitribai Phule Pune Univ, Dept Phys, Pune 411007, Maharashtra, India
[3] Shivaji Univ, Dept Chem, Kolhapur 416004, Maharashtra, India
关键词
Hydrothermal method; Photocatalytic degradation; Salicylic acid; Chemical oxygen demand; REDUCED GRAPHENE OXIDE; ASSISTED PHOTOELECTROCATALYTIC DEGRADATION; TIO2; WO3; SHEETS; FILMS;
D O I
10.1016/j.ultsonch.2019.104849
中图分类号
O42 [声学];
学科分类号
070206 ; 082403 ;
摘要
The current research work deals with the preparation of TiO2 and GO/TiO2 composite by simple, chemical, cost effective hydrothermal method. Graphene oxide (GO) is prepared by modified Hummer's method. Dispersion of GO is achieved by an ultrasonic cleaning bath for 1 h. using a power of 200 W and at a frequency of 40 kHz. The prepared catalyst material is characterized by different characterization techniques. XRD study confirms the prepared material is polycrystalline in nature. The synthesized TiO2 and GO/TiO2 photocatalyst materials are used to study the photocatalytic degradation of salicylic acid under sunlight illumination. GO/TiO2 composite shows superior photocatalytic activity than TiO2. GO/TiO2 composite shows 57% degradation of salicylic acid. Mineralization of salicylic acid is studied using chemical oxygen demand.
引用
收藏
页数:6
相关论文
共 40 条
[1]   UV assisted photoelectrocatalytic degradation of reactive red 152 dye using spray deposited TiO2 thin films [J].
Ali, Tayyab ;
Hunge, Yuvaraj M. ;
Venkatraman, A. .
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2018, 29 (02) :1209-1215
[2]   Molecular Chromophore-Catalyst Assemblies for Solar Fuel Applications [J].
Ashford, Dennis L. ;
Gish, Melissa K. ;
Vannucci, Aaron K. ;
Brennaman, M. Kyle ;
Templeton, Joseph L. ;
Papanikolas, John M. ;
Meyer, Thomas J. .
CHEMICAL REVIEWS, 2015, 115 (23) :13006-13049
[3]  
Basheer C., 2013, J CHEM, V2013
[4]   Photocatalytic activity and stability of TiO2 and WO3 thin films [J].
Carcel, Radu Adrian ;
Andronic, Luminita ;
Duta, Anca .
MATERIALS CHARACTERIZATION, 2012, 70 :68-73
[5]  
Chen Q., J MAT SCI MAT ELECT, V28, P9416
[6]   Bare TiO2 and graphene oxide TiO2 photocatalysts on the degradationof selected pesticides and influence of the water matrix [J].
Cruz, Marta ;
Gomez, Cristina ;
Duran-Valle, Carlos J. ;
Pastrana-Martinez, Luisa M. ;
Faria, Joaquim L. ;
Silva, Adrian M. T. ;
Faraldos, Marisol ;
Bahamonde, Ana .
APPLIED SURFACE SCIENCE, 2017, 416 :1013-1021
[7]   Synthesis of reduced graphene oxide-TiO2 nanoparticle composite systems and its application in hydrogen production [J].
Dubey, Pawan Kumar ;
Tripathi, Prashant ;
Tiwari, R. S. ;
Sinha, A. S. K. ;
Srivastava, O. N. .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2014, 39 (29) :16282-16292
[8]   Synthesis of highly dispersed and versatile anatase TiO2 nanocrystals on graphene sheets with enhanced photocatalytic performance for dye degradation [J].
Gong, Ying ;
Ma, Xiangrong ;
Dang, Rui ;
Liu, Jieying ;
Cao, Ju .
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2017, 28 (24) :18883-18890
[9]   Microstructure and photocatalytic properties of WO3/TiO2 composite films by plasma electrolytic oxidation [J].
He, J. ;
Luo, Q. ;
Cai, Q. Z. ;
Li, X. W. ;
Zhang, D. Q. .
MATERIALS CHEMISTRY AND PHYSICS, 2011, 129 (1-2) :242-248
[10]   Photoelectrocatalytic degradation of diazo dyes on nanostructured WO3 electrodes [J].
Hepel, M ;
Hazelton, S .
ELECTROCHIMICA ACTA, 2005, 50 (25-26) :5278-5291