Femtosecond laser desorption of CO from the Pt(111) surface

被引：27
|
作者：
Cai, L [1 ]
Xiao, XD [1 ]
Loy, MMT [1 ]
机构：
[1] Hong Kong Univ Sci & Technol, Dept Phys, Hong Kong, Hong Kong, Peoples R China
来源：
SURFACE SCIENCE | 2000年 / 464卷 / 2-3期
关键词：
carbon monoxide; laser methods; photon stimulated desorption (PSD); platinum;
D O I：
10.1016/S0039-6028(00)00754-8
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
We report the first study of femtosecond desorption of CO from Pt(111), using 800 nm laser pulses with durations from 125 fs to 1.5 ps. The results for the CO/Pt system are qualitatively similar to other diatomic molecule systems previously studied and can be understood using the electronic friction model. We also studied the CO desorption yield using frequency-chirped laser pulses of the same pulse duration. With the chirping magnitude of ca. 1.5% in our experiment we did not observe any difference between positive and negative chirping. (C) 2000 Elsevier Science B.V. All rights reserved.
引用
收藏
页码：L727 / L731
页数：5
相关论文
共 50 条
  • [1] Desorption of polyatomic molecules from the Pt(111) surface by femtosecond laser radiation
    Cai, L
    Xiao, XD
    Loy, MMT
    JOURNAL OF CHEMICAL PHYSICS, 2001, 115 (20): : 9490 - 9495
  • [2] A restructuring of the CO/Pt(111) surface induced by femtosecond laser pulses?
    Fournier, F
    Zheng, WQ
    Carrez, S
    Dubost, H
    Bourguignon, B
    SURFACE SCIENCE, 2003, 528 (1-3) : 177 - 182
  • [3] FEMTOSECOND LASER-DESORPTION OF MOLECULARLY ADSORBED OXYGEN FROM PT(111)
    KAO, FJ
    BUSCH, DG
    COHEN, D
    DACOSTA, DG
    HO, W
    PHYSICAL REVIEW LETTERS, 1993, 71 (13) : 2094 - 2097
  • [4] Lateral hopping of CO molecules on Pt(111) surface by femtosecond laser pulses
    Hayashi, M.
    Ootsuka, Y.
    Paulsson, M.
    Persson, B. N. J.
    Ueba, H.
    PHYSICAL REVIEW B, 2009, 80 (24)
  • [5] Multicoverage Study of Femtosecond Laser-Induced Desorption of CO from Pd(111)
    Muzas, Alberto S.
    Jimenez, Alfredo Serrano
    Zhang, Yaolong
    Jiang, Bin
    Juaristi, J. Inaki
    Alducin, Maite
    JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2024, 15 (09): : 2587 - 2594
  • [6] Adsorption and desorption of NO and CO on a Pt(111)-Ge surface alloy
    Fukutani, K
    Magkoev, TT
    Murata, Y
    Terakura, K
    SURFACE SCIENCE, 1996, 363 (1-3) : 185 - 194
  • [7] CO DESORPTION AND ADSORPTION ON PT(111)
    WINICUR, DH
    HURST, J
    BECKER, CA
    WHARTON, L
    SURFACE SCIENCE, 1981, 109 (01) : 263 - 275
  • [8] Femtosecond near-infrared laser desorption of multilayer benzene on Pt{111}: spatial origin of hyperthermal desorption
    Arnolds, H
    Rehbein, CEM
    Roberts, G
    Levis, RJ
    King, DA
    CHEMICAL PHYSICS LETTERS, 1999, 314 (5-6) : 389 - 395
  • [9] UV-LASER-INDUCED DESORPTION OF NO FROM PT(111)
    FUKUTANI, K
    MURATA, Y
    SCHWARZWALD, R
    CHUANG, TJ
    SURFACE SCIENCE, 1994, 311 (1-2) : 247 - 256
  • [10] Water desorption from an oxygen covered Pt(111) surface:: Multichannel desorption
    Karlberg, G. S.
    Wahnstrom, G.
    Clay, C.
    Zimbitas, G.
    Hodgson, A.
    JOURNAL OF CHEMICAL PHYSICS, 2006, 124 (20):
12345