Resonant third-order optical nonlinearity in the layered perovskite-type material (C6H13NH3)2PbI4

被引:115
作者
Kondo, T
Iwamoto, S
Hayase, S
Tanaka, K
Ishi, J
Mizuno, M
Ema, K
Ito, R
机构
[1] Univ Tokyo, Fac Engn, Dept Appl Phys, Bunkyo Ku, Tokyo 113, Japan
[2] Sophia Univ, Dept Phys, Chiyoda Ku, Tokyo 102, Japan
关键词
quantum wells; optical properties; nonlinear optics;
D O I
10.1016/S0038-1098(97)10166-1
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The third-order nonlinear optical susceptibility, chi((3))(-omega; omega, -omega, omega), of the layered perovskite-type material (C6H13NH3)(2)PbI4 is measured by a transient four-wave mixing technique using a 200-fs-pulse laser source. The maximum \chi((3))\ value is 1.6 x 10(-6) esu at the lowest-exciton resonance at 8 K. Longitudinal and transverse relaxation times of the excitons are 7 ps and 0.2 ps, respectively. (C) 1998 Elsevier Science Ltd.
引用
收藏
页码:503 / 506
页数:4
相关论文
共 10 条
  • [1] OPTICAL NONLINEARITIES AND PHASE COHERENCE IN CDSE STUDIED BY TRANSIENT 4-WAVE MIXING
    DORNFELD, C
    HVAM, JM
    [J]. IEEE JOURNAL OF QUANTUM ELECTRONICS, 1989, 25 (05) : 904 - 912
  • [2] ISHI J, UNPUB J NONLINEAR OP
  • [3] OPTICAL-PROPERTIES DUE TO ELECTRONIC-TRANSITIONS IN 2-DIMENSIONAL SEMICONDUCTORS (CNH2N + 1NH3)2PBI4
    ISHIHARA, T
    TAKAHASHI, J
    GOTO, T
    [J]. PHYSICAL REVIEW B, 1990, 42 (17): : 11099 - 11107
  • [4] ISHIHARA T, 1995, OPTICAL PROPERTIES L, pCH6
  • [5] MAGNETOOPTICAL STUDY ON EXCITONIC SPECTRA IN (C6H13NH3)2PBI4
    KATAOKA, T
    KONDO, T
    ITO, R
    SASAKI, S
    UCHIDA, K
    MIURA, N
    [J]. PHYSICAL REVIEW B, 1993, 47 (04): : 2010 - 2018
  • [6] KATAOKA T, 1993, THESIS U TOKYO
  • [7] Biexciton lasing in the layered perovskite-type material (C6H13NH3)2PbI4
    Kondo, T
    Azuma, T
    Yuasa, T
    Ito, R
    [J]. SOLID STATE COMMUNICATIONS, 1998, 105 (04) : 253 - 255
  • [8] SYNTHESIS AND CHARACTERIZATION OF [NH2C(I)=NH2](3)MI(5) (M=SN, PB) - STEREOCHEMICAL ACTIVITY IN DIVALENT TIN AND LEAD HALIDES CONTAINING SINGLE [110] PEROVSKITE SHEETS
    WANG, SM
    MITZI, DB
    FEILD, CA
    GULOY, A
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1995, 117 (19) : 5297 - 5302
  • [9] OPTICAL 3RD-HARMONIC GENERATION IN LAYERED PEROVSKITE-TYPE MATERIAL (C10H21NH3)2PBI4
    XU, CQ
    KONDO, T
    SAKAKURA, H
    KUMATA, K
    TAKAHASHI, Y
    ITO, R
    [J]. SOLID STATE COMMUNICATIONS, 1991, 79 (03) : 245 - 248
  • [10] TRANSIENT 4-WAVE MIXING AND COHERENT TRANSIENT OPTICAL PHENOMENA
    YE, PX
    SHEN, YR
    [J]. PHYSICAL REVIEW A, 1982, 25 (04): : 2183 - 2199