Resonant third-order optical nonlinearity in the layered perovskite-type material (C6H13NH3)2PbI4

被引:116
作者
Kondo, T
Iwamoto, S
Hayase, S
Tanaka, K
Ishi, J
Mizuno, M
Ema, K
Ito, R
机构
[1] Univ Tokyo, Fac Engn, Dept Appl Phys, Bunkyo Ku, Tokyo 113, Japan
[2] Sophia Univ, Dept Phys, Chiyoda Ku, Tokyo 102, Japan
关键词
quantum wells; optical properties; nonlinear optics;
D O I
10.1016/S0038-1098(97)10166-1
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The third-order nonlinear optical susceptibility, chi((3))(-omega; omega, -omega, omega), of the layered perovskite-type material (C6H13NH3)(2)PbI4 is measured by a transient four-wave mixing technique using a 200-fs-pulse laser source. The maximum \chi((3))\ value is 1.6 x 10(-6) esu at the lowest-exciton resonance at 8 K. Longitudinal and transverse relaxation times of the excitons are 7 ps and 0.2 ps, respectively. (C) 1998 Elsevier Science Ltd.
引用
收藏
页码:503 / 506
页数:4
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