A new zeolitic lithium aluminum imidazolate framework

被引：3

作者：

Jiang, Guangshen ^{[1
,2
]}

Bon, Volodymyr ^{[2
]}

Xu, Fei ^{[1
,2
]}

Garai, Bikash ^{[2
]}

Zhang, En ^{[2
]}

Senkovska, Irena ^{[2
]}

Poetke, Stephanie ^{[3
]}

Hippauf, Felix ^{[3
]}

Hausdorf, Steffen ^{[2
]}

Paasch, Silvia ^{[4
]}

Brunner, Eike ^{[4
]}

Wang, Hongqiang ^{[1
]}

Kaskel, Stefan ^{[2
,3
]}

机构：

[1] Northwestern Polytech Univ, State Key Lab Solidificat Proc, Sch Mat Sci & Engn, Shaanxi Joint Lab Graphene NPU, Xian 710072, Peoples R China

[2] Tech Univ Dresden, Dept Inorgan Chem, Bergstr 66, D-01062 Dresden, Germany

[3] Fraunhofer Inst Mat & Beam Technol IWS, Winterbergstr 28, D-01277 Dresden, Germany

[4] Tech Univ Dresden, Dept Bioanalyt Chem, Bergstr 66, D-01062 Dresden, Germany

来源：

DALTON TRANSACTIONS | 2021年 / 50卷 / 23期

基金：

中国国家自然科学基金;

关键词：

METAL-ORGANIC FRAMEWORK; THERMAL-STABILITY; GAS-ADSORPTION; ZIF-8; SEPARATION; MEMBRANES;

D O I：

10.1039/d1dt01017d

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

An aliovalent mixed-metal framework DUT-174 [LiAl(2-methylimidazolate)(4)](n), isostructural to ZIF-8, was synthesized from lithium aluminum hydride (LiAlH4) and 2-methylimidazole (2-mImH) through dehydrogenation. Lithium and aluminum cations acting as alternating framework nodes are coordinated tetrahedrally by (2-mIm)(-). DUT-174 has a high specific surface area of 1149 m(2) g(-1) and CO2 uptake of 11.57 mmol g(-1) at 195 K.

引用

页码：7933 / 7937

页数：5

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