Modeling liquid water transport in gas diffusion layers by topologically equivalent pore network

被引:69
|
作者
Luo, Gang
Ji, Yan
Wang, Chao-Yang [1 ]
Sinha, Puneet K.
机构
[1] Penn State Univ, Electrochem Engine Ctr ECEC, University Pk, PA 16802 USA
关键词
Polymer electrolyte fuel cells (PEFC); Topologically equivalent pore network (TEPN); Gas diffusion layer (GDL); Relative permeability; Liquid water distribution; MEMBRANE FUEL-CELLS; 2-PHASE FLOW; BEHAVIOR;
D O I
10.1016/j.electacta.2010.04.078
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
A topologically equivalent pore network (TEPN) model is developed for the first time to extract pore networks directly from gas diffusion layer (GDL) microstructures and thus account for all structural features of a GDL material. A generic framework of TEPN modeling is presented to design GDL structures that enable improved water management. With TEPNs used as input to a two-phase flow simulator, constitutive relations and steady-state liquid saturation profiles for carbon paper and carbon cloth are obtained and reported in this work. The results indicate a strong influence of the GDL morphology on water transport characteristics, which helps unravel the structure-performance relationship for GDLs. (C) 2010 Elsevier Ltd. All rights reserved.
引用
收藏
页码:5332 / 5341
页数:10
相关论文
共 50 条
  • [21] Effect of compression of microporous and gas diffusion layers on liquid water transport of PEMFC with interdigitated flow field by Lattice Boltzmann method
    Moslemi, Mehdi
    Javaherdeh, Kourosh
    Ashorynejad, Hamid Reza
    COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2022, 642
  • [22] Stochastic Aspects of Mass Transport in Gas Diffusion Layers
    Froning, Dieter
    Gaiselmann, Gerd
    Reimer, Uwe
    Brinkmann, Jan
    Schmidt, Volker
    Lehnert, Werner
    TRANSPORT IN POROUS MEDIA, 2014, 103 (03) : 469 - 495
  • [23] Transport Phenomena in Carbon Paper Gas Diffusion Layers
    Didari, Sima
    Harris, Tequila A. L.
    Huang, Wei
    Tessier, Sean M.
    Wang, Yan
    POLYMER ELECTROLYTE FUEL CELLS 11, 2011, 41 (01): : 499 - 512
  • [24] An integrated model of the water transport in nonuniform compressed gas diffusion layers for PEMFC<bold> </bold>
    Xu, Yifan
    Qiu, Diankai
    Yi, Peiyun
    Lan, Shuhuai
    Peng, Linfa
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2019, 44 (26) : 13777 - 13785
  • [25] Pore network modeling of two-phase flow in a liquid-(disconnected) gas system
    Bravo, Maria C.
    Araujo, Mariela
    Lago, Marcelo E.
    PHYSICA A-STATISTICAL MECHANICS AND ITS APPLICATIONS, 2007, 375 (01) : 1 - 17
  • [26] Pore-network simulations of two-phase flow in a thin porous layer of mixed wettability: Application to water transport in gas diffusion layers of proton exchange membrane fuel cells
    Kuttanikkad, S. Pulloor
    Prat, M.
    Pauchet, J.
    JOURNAL OF POWER SOURCES, 2011, 196 (03) : 1145 - 1155
  • [27] Random Pore Network Modeling of Fibrous PEMFC Gas Diffusion Media Using Voronoi and Delaunay Tessellations
    Gostick, Jeff T.
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2013, 160 (08) : F731 - F743
  • [28] Multi-scaled pore network modeling of gas-water flow in shale formations
    Wang, Xiukun
    Sheng, James J.
    JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING, 2019, 177 : 899 - 908
  • [29] Estimation of Relative Transport Properties in Porous Transport Layers Using Pore-Scale and Pore-Network Simulations
    Jung, Seongyeop
    Sabharwal, Mayank
    Jarauta, Alex
    Wei, Fei
    Gingras, Murray
    Gostick, Jeff
    Secanell, Marc
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2021, 168 (06)
  • [30] Influences of the perforation on effective transport properties of gas diffusion layers
    Fang, Wen-Zhen
    Tang, Yu-Qing
    Chen, Li
    Kang, Qin-Jun
    Tao, Wen-Quan
    INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2018, 126 : 243 - 255