Correlated Electrons in Optically Tunable Quantum Dots: Building an Electron Dimer Molecule

被引:37
作者
Singha, Achintya [1 ,2 ]
Pellegrini, Vittorio [1 ,2 ]
Pinczuk, Aron [3 ,4 ,5 ]
Pfeiffer, Loren N. [6 ,8 ]
West, Ken W. [6 ,8 ]
Rontani, Massimo [7 ]
机构
[1] CNR, NEST, Ist Nanosci, I-56127 Pisa, Italy
[2] Scuola Normale Super Pisa, I-56127 Pisa, Italy
[3] Columbia Univ, Dept Appl Phys, New York, NY 10027 USA
[4] Columbia Univ, Dept Appl Math, New York, NY 10027 USA
[5] Columbia Univ, Dept Phys, New York, NY 10027 USA
[6] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA
[7] CNR, Ist Nanosci, S3, I-41125 Modena, Italy
[8] Alcatel Lucent, Bell Labs, Murray Hill, NJ 07974 USA
基金
美国国家科学基金会;
关键词
MAGNETIC-FIELD; SPECTROSCOPY; EXCITATIONS; SCATTERING; MOTION;
D O I
10.1103/PhysRevLett.104.246802
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We observe the low-lying excitations of a molecular dimer formed by two electrons in a GaAs semiconductor quantum dot in which the number of confined electrons is tuned by optical illumination. By employing inelastic light scattering we identify the intershell excitations in the one-electron regime and the distinct spin and charge modes in the interacting few-body configuration. In the case of two electrons, a comparison with configuration-interaction calculations allows us to link the observed excitations with the breathing mode of the molecular dimer and to determine the singlet-triplet energy splitting.
引用
收藏
页数:4
相关论文
共 28 条
[1]   Spectroscopy of few-electron collective excitations in charge-tunable artificial atoms -: art. no. 257401 [J].
Brocke, T ;
Bootsmann, MT ;
Tews, M ;
Wunsch, B ;
Pfannkuche, D ;
Heyn, C ;
Hansen, W ;
Heitmann, D ;
Schüller, C .
PHYSICAL REVIEW LETTERS, 2003, 91 (25)
[2]   ELECTRONIC-STRUCTURE OF ULTRASMALL QUANTUM-WELL BOXES [J].
BRYANT, GW .
PHYSICAL REVIEW LETTERS, 1987, 59 (10) :1140-1143
[3]   Coupled quantum dots as quantum gates [J].
Burkard, G ;
Loss, D ;
DiVincenzo, DP .
PHYSICAL REVIEW B, 1999, 59 (03) :2070-2078
[4]   SPECTROSCOPY OF QUANTUM LEVELS IN CHARGE-TUNABLE INGAAS QUANTUM DOTS [J].
DREXLER, H ;
LEONARD, D ;
HANSEN, W ;
KOTTHAUS, JP ;
PETROFF, PM .
PHYSICAL REVIEW LETTERS, 1994, 73 (16) :2252-2255
[5]   Crossover from fermi liquid to Wigner molecule behavior in quantum dots [J].
Egger, R ;
Häusler, W ;
Mak, CH ;
Grabert, H .
PHYSICAL REVIEW LETTERS, 1999, 82 (16) :3320-3323
[6]   Excitation spectrum of two correlated electrons in a lateral quantum dot with negligible Zeeman splitting [J].
Ellenberger, C ;
Ihn, T ;
Yannouleas, C ;
Landman, U ;
Ensslin, K ;
Driscoll, D ;
Gossard, AC .
PHYSICAL REVIEW LETTERS, 2006, 96 (12) :1-4
[7]   Evidence of correlation in spin excitations of few-electron quantum dots -: art. no. 266806 [J].
García, CP ;
Pellegrini, V ;
Pinczuk, A ;
Rontani, M ;
Goldoni, G ;
Molinari, E ;
Dennis, BS ;
Pfeiffer, LN ;
West, KW .
PHYSICAL REVIEW LETTERS, 2005, 95 (26)
[8]   Correlation-induced inhomogeneity in circular quantumdots [J].
Ghosal, Amit ;
Guclu, A. D. ;
Umrigar, C. J. ;
Ullmo, Denis ;
Baranger, Harold U. .
NATURE PHYSICS, 2006, 2 (05) :336-340
[9]   Spins in few-electron quantum dots [J].
Hanson, R. ;
Kouwenhoven, L. P. ;
Petta, J. R. ;
Tarucha, S. ;
Vandersypen, L. M. K. .
REVIEWS OF MODERN PHYSICS, 2007, 79 (04) :1217-1265
[10]   A molecular state of correlated electrons in a quantum dot [J].
Kalliakos, Sokratis ;
Rontani, Massimo ;
Pellegrini, Vittorio ;
Garcia, Cesar Pascual ;
Pinczuk, Aron ;
Goldoni, Guido ;
Molinari, Elisa ;
Pfeiffer, Loren N. ;
West, Ken W. .
NATURE PHYSICS, 2008, 4 (06) :467-471