High-throughput screening of heterogeneous catalyst under pressurized conditions - Optimization of Cu-Mn oxide catalyst for methanol synthesis

被引:0
|
作者
Omata, K [1 ]
Ishiguro, G [1 ]
Yamada, M [1 ]
机构
[1] Tohoku Univ, Grad Sch Engn, Dept Appl Chem, Aoba Ku, Sendai, Miyagi 9808579, Japan
来源
SEKIYU GAKKAISHI-JOURNAL OF THE JAPAN PETROLEUM INSTITUTE | 2000年 / 43卷 / 04期
关键词
reactor; activity; mixed oxide catalyst; methanol; combinatorial chemistry; high-throughput screening;
D O I
暂无
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
High-throughput screening was performed to optimize the Cu/Mn ratio of Cu-Mn oxide catalyst for methanol synthesis from syngas at 1 MPa and 523 K. The autoclave equipped with twelve catalyst beds was connected to a conventional high-pressure gas flow apparatus. Identical temperature and identical space velocity over the 12 catalyst beds was ensured. The catalyst showed the same activity as that of the catalyst used in the conventional test, indicating the possibility of high efficiency catalyst screening under conventional testing conditions.
引用
收藏
页码:317 / 319
页数:3
相关论文
共 40 条
  • [31] Design of Cu-Zn-Al-Sc oxide catalyst for methanol synthesis using genetic algorithm based on radial basis function network as the evaluation function
    Omata, K
    Umegaki, T
    Watanabe, Y
    Nukui, N
    Yamada, M
    JOURNAL OF THE JAPAN PETROLEUM INSTITUTE, 2003, 46 (03) : 189 - 195
  • [32] Development of a high performance Cu-based ternary oxide catalyst for oxidative steam reforming of methanol using an artificial neural network
    Umegaki, Tetsuo
    Masuda, Akihiro
    Omata, Kohji
    Yamada, Muneyoshi
    APPLIED CATALYSIS A-GENERAL, 2008, 351 (02) : 210 - 216
  • [33] Palladium supported on zinc oxide nanoparticles: Synthesis, characterization, and application as heterogeneous catalyst for Mizoroki-Heck and Sonogashira reactions under ligand-free and air atmosphere conditions
    Hosseini-Sarvari, Mona
    Razmi, Zahra
    Doroodmand, Mohammad Mehdi
    APPLIED CATALYSIS A-GENERAL, 2014, 475 : 477 - 486
  • [34] High-Throughput Reaction Optimisation and Activity Screening of Ferrocene-Based Lewis Acid-Catalyst Complexes by Using Continuous-Flow Reaction Detection Mass Spectrometry
    Martha, Cornelius T.
    Heemskerk, Anton
    Hoogendoorn, Jan-Carel
    Elders, Niels
    Niessen, Wilfried M. A.
    Orru, Romano V. A.
    Irth, Hubertus
    CHEMISTRY-A EUROPEAN JOURNAL, 2009, 15 (30) : 7368 - 7375
  • [35] Reaction Analyses Based on Quaternary Metal/Metal Oxide Catalyst Testing in Micro-Structured Reactors Using Combinatorial High-Throughput Methods for Power-to-Gas Applications
    Pfeifer, Mirko
    Schwarz, Thomas
    Cao, Pengfei
    Stoewe, Klaus
    CATALYSTS, 2021, 11 (01) : 1 - 18
  • [36] Mg,Al-mixed oxide system: Synthesis under hydrothermal conditions.) physico-chemical characterisation and application as an efficient catalyst for imidazole methylation
    Grabowska, H
    Zawadzki, M
    Syper, L
    Mista, W
    APPLIED CATALYSIS A-GENERAL, 2005, 292 : 208 - 214
  • [37] Catalysts screening, optimization and mechanism studies of dimethylhexane-1,6-dicarbamate synthesis from 1,6-hexanediamine and dimethyl carbonate over Mn(OAc)2 catalyst
    Zhao, Liyan
    He, Peng
    Wang, Liguo
    Ammar, Muhammad
    Cao, Yan
    Li, Huiquan
    CATALYSIS TODAY, 2017, 281 : 392 - 401
  • [38] Optimization of methanol synthesis reaction on Cu/ZnO/Al2O3/ZrO2 catalyst using genetic algorithm: Maximization of the synergetic effect by the optimal CO2 fraction
    Lim, Hye-Won
    Jun, Hye Jin
    Park, Myung-June
    Kim, Hyo-Sik
    Bae, Jong Wook
    Ha, Kyoung-Su
    Chae, Ho-Jeong
    Jun, Ki-Won
    KOREAN JOURNAL OF CHEMICAL ENGINEERING, 2010, 27 (06) : 1760 - 1767
  • [39] Optimization of methanol synthesis reaction on Cu/ZnO/Al2O3/ZrO2 catalyst using genetic algorithm: Maximization of the synergetic effect by the optimal CO2 fraction
    Hye-Won Lim
    Hye Jin Jun
    Myung-June Park
    Hyo-Sik Kim
    Jong Wook Bae
    Kyoung-Su Ha
    Ho-Jeong Chae
    Ki-Won Jun
    Korean Journal of Chemical Engineering, 2010, 27 : 1760 - 1767
  • [40] Design and characterization of Dendrimer of MNPs as a novel, heterogeneous and reusable nanomagnetic organometallic catalyst for one-pot synthesis of hydroxyl naphthalene-1,4-dione derivatives under solvent-free conditions
    Mollazehi, Fouziyeh
    Shaterian, Hamid Reza
    APPLIED ORGANOMETALLIC CHEMISTRY, 2018, 32 (03)