Quantification of vehicle fleet PM10 particulate matter emission factors from exhaust and non-exhaust sources using tunnel measurement techniques

被引:93
作者
Lawrence, Samantha [1 ]
Sokhi, Ranjeet [1 ]
Ravindra, Khaiwal [2 ]
机构
[1] Univ Hertfordshire, CAIR, Hatfield AL10 9AB, Herts, England
[2] PGIMER, Sch Publ Hlth, Chandigarh 160012, India
基金
英国自然环境研究理事会;
关键词
Non-exhaust; Emission factors; PM10 and PM2.5; Brakewear Road surface; Re-suspension; Tukey mean-difference (Bland and Altman) plot; POLYCYCLIC AROMATIC-HYDROCARBONS; ROAD DUST; PARTICLE EMISSIONS; FINE; PM2.5; RESUSPENSION; AEROSOL; METALS; MODEL; RATES;
D O I
10.1016/j.envpol.2016.01.011
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Road tunnels act like large laboratories; they provide an excellent environment to quantify atmospheric particles emission factors from exhaust and non-exhaust sources due to their known boundary conditions. Current work compares the High Volume, Dichotomous Stacked Filter Unit and Partisol Air Sampler for coarse, PM10 and PM25 particle concentration measurement and found that they do not differ significantly (p = 95%). PM2.5 fraction contributes 66% of PM-m proportions and significantly influenced by traffic (turbulence) and meteorological conditions. Mass emission factors for PM10 varies from 21.3 +/- 1.9 to 28.8 +/- 3.4 mg/vkm and composed of Motorcycle (0.0003-0.001 mg/vkm), Cars (26.1-33.4 mg/vkm), LDVs (2.4-3.0 mg/vkm), HDVs (2.2-2.8 mg/vkm) and Buses (0.1 mg/vkm). Based on Lawrence et al. (2013), source apportionment modelling, the PM10 emission of brake wear (3.8-4.4 mg/vkm), petrol exhaust (3.9-4.5 mg/vkm), diesel exhaust (7.2-8.3 mg/vkm), re-suspension (9-10.4 mg/vkm), road surface wear (3.9-4.5 mg/vkm), and unexplained (7.2 mg/vkm) were also calculated. The current study determined that the combined non-exhaust fleet PM10 emission factor (16.7-19.3 mg/vkm) are higher than the combined exhaust emission factor (11.1-12.8 mg/vkm). Thus, highlight the significance of non-exhaust emissions and the need for legislation and abatement strategies to reduce their contributions to ambient PM concentrations. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:419 / 428
页数:10
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