Automated polarization-dependent multidimensional coherent spectroscopy phased using transient absorption

被引：3
作者：
Wahlstrand, J. K. [1 ]
Wernsing, G. M. [1 ,2 ]
Paul, J. [1 ,3 ]
Bristow, A. D. [1 ,3 ]
机构：
[1] NIST, Nanoscale Device Characterizat Div, Gaithersburg, MD 20899 USA
[2] Worcester Polytech Inst, Elect & Comp Engn, Worcester, MA 01609 USA
[3] West Virginia Univ, Dept Phys & Astron, Morgantown, WV 26506 USA
来源：
OPTICS EXPRESS | 2019年 / 27卷 / 22期
关键词：
FOURIER-TRANSFORM SPECTROSCOPY;
D O I：
10.1364/OE.27.031790
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
An experimental apparatus is described for multidimensional optical spectroscopy with fully automated polarization control, based on liquid crystal variable retarders. Polarization dependence of rephasing two-dimensional coherent spectra are measured in a single scan, with absolute phasing performed for all polarization configurations through a single automated auxiliary measurement at the beginning of the scan. A factor of three improvement in acquisition time is demonstrated, compared to the apparatus without automated polarization control. Results are presented for a GaAs quantum well sample and an InGaAs quantum well embedded in a microcavity. (C) 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
引用
收藏
页码：31790 / 31799
页数：10
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