Microscope Analysis of Au-Pd/TiO2 Glycerol Oxidation Catalysts Prepared by Deposition-Precipitation Method

被引:20
|
作者
Mimura, Naoki [1 ]
Hiyoshi, Norihito [1 ]
Date, Masakazu [2 ]
Fujitani, Tadahiro [3 ]
Dumeignil, Franck [4 ,5 ]
机构
[1] Natl Inst Adv Ind Sci & Technol, Res Ctr Compact Chem Syst, Miyagino Ku, Sendai, Miyagi 9838551, Japan
[2] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan
[3] Natl Inst Adv Ind Sci & Technol, Res Inst Innovat Sustainable Chem, Tsukuba, Ibaraki 3058565, Japan
[4] Univ Lille Sci & Technol 1, UMR CNRS 8181, UCCS, F-59655 Villeneuve Dascq, France
[5] Maison Univ, Inst Univ France, F-75005 Paris, France
基金
日本学术振兴会;
关键词
Nanoparticle catalyst; Glycerol oxidation; High-resolution EDS analysis; LIQUID-PHASE OXIDATION; SELECTIVE OXIDATION; BIMETALLIC CATALYSTS; AU; PD; NANOPARTICLES; TEMPERATURE; OXYGEN; MONO; CO;
D O I
10.1007/s10562-014-1382-6
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Gold-palladium bimetallic nanoparticle catalysts prepared by a deposition-precipitation method were effective for aerobic oxidation of glycerol to carboxylic acids. The role of palladium was to suppress C-C bond cleavage that is responsible for the formation of C2 by-product molecules. The nanoparticles were observed by microscope techniques, which further enabled characterizing the respective locations of Au and Pd within the particles.
引用
收藏
页码:2167 / 2175
页数:9
相关论文
共 50 条
  • [1] Microscope Analysis of Au–Pd/TiO2 Glycerol Oxidation Catalysts Prepared by Deposition–Precipitation Method
    Naoki Mimura
    Norihito Hiyoshi
    Masakazu Daté
    Tadahiro Fujitani
    Franck Dumeignil
    Catalysis Letters, 2014, 144 : 2167 - 2175
  • [2] Catalytic Performance and Reaction Mechanisms of Ethyl Acetate Oxidation over the Au-Pd/TiO2 Catalysts
    Bao, Minming
    Liu, Yuxi
    Deng, Jiguang
    Jing, Lin
    Hou, Zhiquan
    Wang, Zhiwei
    Wei, Lu
    Yu, Xiaohui
    Dai, Hongxing
    CATALYSTS, 2023, 13 (04)
  • [3] Improved activity and stability in CO oxidation of bimetallic Au-Cu/TiO2 catalysts prepared by deposition-precipitation with urea
    Sandoval, Alberto
    Louis, Catherine
    Zanella, Rodolfo
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2013, 140 : 363 - 377
  • [4] Bimetallic Au-Ag/TiO2 catalyst prepared by deposition-precipitation: High activity and stability in CO oxidation
    Sandoval, Alberto
    Aguilar, Antonio
    Louis, Catherine
    Traverse, Agnes
    Zanella, Rodolfo
    JOURNAL OF CATALYSIS, 2011, 281 (01) : 40 - 49
  • [5] Synthesis and characterization of Au-Pd/SiO2 bimetallic catalysts prepared by electroless deposition
    Rebelli, Jayakiran
    Detwiler, Michael
    Ma, Shuguo
    Williams, Christopher T.
    Monnier, John R.
    JOURNAL OF CATALYSIS, 2010, 270 (02) : 224 - 233
  • [6] Product Inhibition in Glycerol Oxidation over Au/TiO2 Catalysts Quantified by NMR Relaxation
    D'Agostino, Carmine
    Armstrong, Robert D.
    Hutchings, Graham J.
    Gladden, Lynn F.
    ACS CATALYSIS, 2018, 8 (08): : 7334 - 7339
  • [7] The liquid-phase hydrogenation of 1-heptyne over Pd-Au/TiO2 catalysts prepared by the combination of incipient wetness impregnation and deposition-precipitation
    Kittisakmontree, Prathan
    Pongthawornsakun, Boontida
    Yoshida, Hiroshi
    Fujita, Shin-ichiro
    Arai, Masahiko
    Panpranot, Joongjai
    JOURNAL OF CATALYSIS, 2013, 297 : 155 - 164
  • [8] Selective hydrogenation of 1,3-butadiene over bimetallic Au-Ni/TiO2 catalysts prepared by deposition-precipitation with urea
    Aguilar-Tapia, Antonio
    Delannoy, Laurent
    Louis, Catherine
    Han, Chang Wan
    Ortalan, Volkan
    Zanella, Rodolfo
    JOURNAL OF CATALYSIS, 2016, 344 : 515 - 523
  • [9] Oxidation of cinnamyl alcohol using bimetallic Au-Pd/TiO2 catalysts: a deactivation study in a continuous flow packed bed microreactor
    Wu, Gaowei
    Brett, Gemma L.
    Cao, Enhong
    Constantinou, Achilleas
    Ellis, Peter
    Kuhn, Simon
    Hutchings, Graham J.
    Bethell, Donald
    Gavriilidis, Asterios
    CATALYSIS SCIENCE & TECHNOLOGY, 2016, 6 (13) : 4749 - 4758
  • [10] Synergistic effect of bimetallic Au-Pd supported on ceria-zirconia mixed oxide catalysts for selective oxidation of glycerol
    Olmos, Carol M.
    Chinchilla, Lidia E.
    Rodrigues, Elodie G.
    Delgado, Juan J.
    Hungria, Ana B.
    Blanco, Ginesa
    Pereira, Manuel F. R.
    Orfao, Jose J. M.
    Calvino, Jose J.
    Chen, Xiaowei
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2016, 197 : 222 - 235