Smoothing and coherent structure formation in organic-organic heterostructure growth

被引:25
作者
Hinderhofer, A. [1 ]
Gerlach, A. [1 ]
Kowarik, S. [1 ,2 ]
Zontone, F. [3 ]
Krug, J. [4 ]
Schreiber, F. [1 ]
机构
[1] Univ Tubingen, Inst Angew Phys, D-72076 Tubingen, Germany
[2] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
[3] European Synchrotron Radiat Facil, F-38043 Grenoble 9, France
[4] Univ Cologne, Inst Theoret Phys, D-50937 Cologne, Germany
关键词
THIN-FILMS; ROUGHNESS; DYNAMICS; ORDER;
D O I
10.1209/0295-5075/91/56002
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We use in situ real-time X-ray reflectivity and complementary atomic force microscopy to monitor crystallinity and roughness evolution during growth of organic heterostructures, i.e. perfluoropentacene (PFP) on diindenoperylene (DIP) and pentacene (PEN) on PFP. For both systems, surface smoothing during thermal evaporation of the second material on top of the first is observed. The smoothing can be rationalized by a, compared to homoepitaxy, lowered step edge barrier for one species diffusing on the other. In addition, we find an exceptionally well-ordered interface for PEN-on-PFP growth and PEN growth with anomalously low roughening, along with coherent scattering over the entire thickness. Copyright (C) EPLA, 2010
引用
收藏
页数:5
相关论文
共 23 条
  • [1] [Anonymous], 2004, ISLAND MOUNDS ATOMS, DOI DOI 10.1007/978-3-642-18672-1
  • [2] Nonmonotonic roughness evolution in unstable growth
    Castellano, C
    Krug, J
    [J]. PHYSICAL REVIEW B, 2000, 62 (04) : 2879 - 2888
  • [3] Quantification of line-edge roughness of photoresists. II. Scaling and fractal analysis and the best roughness descriptors
    Constantoudis, V
    Patsis, GP
    Tserepi, A
    Gogolides, E
    [J]. JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B, 2003, 21 (03): : 1019 - 1026
  • [4] Rapid roughening in thin film growth of an organic semiconductor (diindenoperylene) -: art. no. 016104
    Dürr, AC
    Schreiber, F
    Ritley, KA
    Kruppa, V
    Krug, J
    Dosch, H
    Struth, B
    [J]. PHYSICAL REVIEW LETTERS, 2003, 90 (01) : 4
  • [5] High structural order in thin films of the organic semiconductor diindenoperylene
    Dürr, AC
    Schreiber, F
    Münch, M
    Karl, N
    Krause, B
    Kruppa, V
    Dosch, H
    [J]. APPLIED PHYSICS LETTERS, 2002, 81 (12) : 2276 - 2278
  • [6] Ehrlich-Schwoebel effect for organic molecules: Direct calculation of the step-edge barrier using empirical potentials
    Fendrich, M.
    Krug, J.
    [J]. PHYSICAL REVIEW B, 2007, 76 (12)
  • [7] Unstable growth on rough surfaces
    Gyure, MF
    Zinck, JJ
    Ratsch, C
    Vvedensky, DD
    [J]. PHYSICAL REVIEW LETTERS, 1998, 81 (22) : 4931 - 4934
  • [8] Growth dynamics of pentacene thin films
    Heringdorf, FJMZ
    Reuter, MC
    Tromp, RM
    [J]. NATURE, 2001, 412 (6846) : 517 - 520
  • [9] Optical properties of pentacene and perfluoropentacene thin films
    Hinderhofer, Alexander
    Heinemeyer, Ute
    Gerlach, Alexander
    Kowarik, Stefan
    Jacobs, Robert M. J.
    Sakamoto, Youichi
    Suzuki, Toshiyasu
    Schreiber, Frank
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2007, 127 (19)
  • [10] Characterization of step-edge barriers in organic thin-film growth
    Hlawacek, Gregor
    Puschnig, Peter
    Frank, Paul
    Winkler, Adolf
    Ambrosch-Draxl, Claudia
    Teichert, Christian
    [J]. SCIENCE, 2008, 321 (5885) : 108 - 111