Study of electrical and magnetic properties of Ni-Zn-Mg ferrite system

Polycrystalline nickel-zinc ferrites of chemical formula Ni0.65-xMgxZn0.35Fe2O4 (x = 0.00 to 0.2 in steps of 0.04) have been prepared by conventional ceramic technique. Calcination and sintering of all samples have been carried out in air atmosphere at 950 degrees C and 1250 degrees C, respectively, followed by natural cooling to room temperature. All the samples were characterized by the X-ray diffraction (XRD) for structure determination. These samples were then investigated for their magnetic and electric properties, including saturation magnetization, Curie temperature, initial permeability measurements and DC electrical resistivity. Porosity was decreased drastically from 15% to 5% showed better quality of the sintered samples. There were increments in initial permeability and DC electrical resistivity throughout the series of samples. Variations in the observed properties as a function of magnesium concentration have been discussed in light of the existing understanding.