Continuous separation of oil from water surface by a novel tubular unit based on graphene coated polyurethane sponge

被引:13
作者
Zhang, Tai [1 ]
Xiao, Changfa [1 ,2 ,3 ]
Zhao, Jian [1 ]
Chen, Kaikai [1 ]
Hao, Junqiang [1 ]
Ji, Dawei [1 ]
机构
[1] Tianjin Polytech Univ, Sch Text, State Key Lab Separat Membranes & Membrane Proc, Natl Ctr Int Joint Res Separat Membranes, Tianjin 300387, Peoples R China
[2] Tianjin Polytech Univ, Sch Text, Tianjin 300387, Peoples R China
[3] Tianjin Polytech Univ, State Key Lab Separat Membranes & Membrane Proc, Tianjin 300387, Peoples R China
基金
中国国家自然科学基金;
关键词
continuous oil-water separation; graphene; polyurethane sponge; tubular unit; EFFICIENT OIL/WATER SEPARATION; ACTIVATED CARBON; SPILL CLEANUP; REMOVAL; SORBENT; PERFORMANCE; ABSORPTION; NANOTUBE;
D O I
10.1002/pat.4343
中图分类号
O63 [高分子化学(高聚物)];
学科分类号
070305 ; 080501 ; 081704 ;
摘要
We develop a new strategy for the continuous separation of oil from water surface using a novel tubular unit based on graphene coated polyurethane (P-GEPU) sponge, and the P-GEPU sponge was fabricated by a simple dip-coating method; the as-prepared sponges could adsorb different kinds of oil and organic liquids while repelling water. Moreover, the tubular unit was assembled by wrapping the P-GEPU sponge on a porous PU hollow tube and combined with the accessories including pipes and joints. The tubular unit could float on the surface of water, and a continuous oil collection from water surface through vacuum pressure could be fulfilled, showing a high oil-water separation efficiency (>96%). Finally, oil-water separation efficiency remains above 93% after 10cycles, exhibiting excellent reusability. In addition, our findings are easily scaled up, showing a great promise for large-scale oil spill remediation.
引用
收藏
页码:2317 / 2326
页数:10
相关论文
共 35 条
  • [1] Porous materials for oil spill cleanup: A review of synthesis and absorbing properties
    Adebajo, MO
    Frost, RL
    Kloprogge, JT
    Carmody, O
    Kokot, S
    [J]. JOURNAL OF POROUS MATERIALS, 2003, 10 (03) : 159 - 170
  • [2] Residual oil and suspended solid removal using natural adsorbents chitosan, bentonite and activated carbon: A comparative study
    Ahmad, AL
    Sumathi, S
    Hameed, BH
    [J]. CHEMICAL ENGINEERING JOURNAL, 2005, 108 (1-2) : 179 - 185
  • [3] A sustainable approach to controlling oil spills
    Al-Majed, Abdul Aziz
    Adebayo, Abdulrauf Rasheed
    Hossain, M. Enamul
    [J]. JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2012, 113 : 213 - 227
  • [4] Aerostat Sampling of PCDD/PCDF Emissions from the Gulf Oil Spill In Situ Burns
    Aurell, Johanna
    Gullett, Brian K.
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2010, 44 (24) : 9431 - 9437
  • [5] Oil spill cleanup from sea water by sorbent materials
    Bayat, A
    Aghamiri, SF
    Moheb, A
    Vakili-Nezhaad, GR
    [J]. CHEMICAL ENGINEERING & TECHNOLOGY, 2005, 28 (12) : 1525 - 1528
  • [6] Bi HC, 2014, J MATER CHEM A, V2, P1652, DOI [10.1039/c3ta14112h, 10.1039/c3ta14112]
  • [7] Improved mechanical oil spill recovery using an optimized geometry for the skimmer surface
    Broje, Victoria
    Keller, Arturo A.
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2006, 40 (24) : 7914 - 7918
  • [8] Magnetically Driven Floating Foams for the Removal of Oil Contaminants from Water
    Calcagnile, Paola
    Fragouli, Despina
    Bayer, Ilker S.
    Anyfantis, George C.
    Martiradonna, Luigi
    Cozzoli, P. Davide
    Cingolani, Roberto
    Athanassiou, Athanassia
    [J]. ACS NANO, 2012, 6 (06) : 5413 - 5419
  • [9] Mussel-Inspired Chemistry and Michael Addition Reaction for Efficient Oil/Water Separation
    Cao, Yingze
    Zhang, Xiaoyong
    Tao, Lei
    Li, Kan
    Xue, Zhongxin
    Feng, Lin
    Wei, Yen
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2013, 5 (10) : 4438 - 4442
  • [10] Evaluation of Butyl Rubber as Sorbent Material for the Removal of Oil and Polycyclic Aromatic Hydrocarbons from Seawater
    Ceylan, Deniz
    Dogu, Saadet
    Karacik, Burak
    Yakan, Sevil D.
    Okay, Oya S.
    Okay, Oguz
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2009, 43 (10) : 3846 - 3852