Optical Second Harmonic Generation of Single Metallic Nanoparticles Embedded in a Homogeneous Medium

被引：221
|
作者：
Butet, Jeremy [1 ]
Duboisset, Julien [1 ]
Bachelier, Guillaume [1 ]
Russier-Antoine, Isabelle [1 ]
Benichou, Emmanuel [1 ]
Jonin, Christian [1 ]
Brevet, Pierre-Francois [1 ]
机构：
[1] Univ Lyon 1, Spectrometrie Ion & Mol Lab, CNRS, UMR 5579, F-69622 Villeurbanne, France
来源：
NANO LETTERS | 2010年 / 10卷 / 05期
关键词：
Single nanoparticle; gold; plasmonics; nonlinear optics; second harmonic generation; finite element method simulation; HYPER-RAYLEIGH-SCATTERING; GOLD NANOPARTICLES; COPPER NANOPARTICLES; MOLECULE DETECTION; NANODIMERS; RESPONSES; LIMIT;
D O I：
10.1021/nl1000949
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
We report the optical second harmonic generation from individual 150 nm diameter gold nanoparticles dispersed in gelatin. The quadratic hyperpolarizability of the particles is determined and the input polarization dependence of the second harmonic intensity obtained. These results are found in excellent agreement with ensemble measurements and finite element simulations. These results open up new perspectives for the investigation of the nonlinear optical properties of noble metal nanoparticles.
引用
收藏
页码：1717 / 1721
页数：5
相关论文
共 50 条
  • [1] Second Harmonic Generation of Single Metallic Nanoparticles
    Butet, J.
    Bachelier, G.
    Duboisset, J.
    Bertorelle, F.
    Russier-Antoine, I.
    Jonin, Ch
    Benichou, E.
    Brevet, P. F.
    SINGLE MOLECULE SPECTROSCOPY AND IMAGING IV, 2011, 7905
  • [2] Three-dimensional mapping of single gold nanoparticles embedded in a homogeneous transparent matrix using optical second-harmonic generation
    Butet, Jeremy
    Bachelier, Guillaume
    Duboisset, Julien
    Bertorelle, Franck
    Russier-Antoine, Isabelle
    Jonin, Christian
    Benichou, Emmanuel
    Brevet, Pierre-Francois
    OPTICS EXPRESS, 2010, 18 (21): : 22314 - 22323
  • [3] Multipolar Second Harmonic Generation from Metallic Nanoparticles
    Butet, J.
    Bachelier, G.
    Russier-Antoine, I.
    Jonin, Ch.
    Benichou, E.
    Brevet, P. F.
    PROCEEDINGS OF THE INTERNATIONAL CONFERENCE OF COMPUTATIONAL METHODS IN SCIENCES AND ENGINEERING 2010 (ICCMSE-2010), 2015, 1642 : 509 - 513
  • [4] Multipolar Second Harmonic Generation from Metallic Nanoparticles
    Butet, J.
    Bachelier, G.
    Russier-Antoine, I.
    Jonin, Ch.
    Benichou, E.
    Brevet, P. F.
    PHOTONIC AND PHONONIC PROPERTIES OF ENGINEERED NANOSTRUCTURES, 2011, 7946
  • [5] Sensing with Multipolar Second Harmonic Generation from Spherical Metallic Nanoparticles
    Butet, Jeremy
    Russier-Antoine, Isabelle
    Jonin, Christian
    Lascoux, Noelle
    Benichou, Emmanuel
    Brevet, Pierre-Francois
    NANO LETTERS, 2012, 12 (03) : 1697 - 1701
  • [6] Optical Second Harmonic Generation in Plasmonic Nanostructures: From Fundamental Principles to Advanced Applications
    Butet, Jeremy
    Brevet, Pierre-Francois
    Martin, Olivier J. F.
    ACS NANO, 2015, 9 (11) : 10545 - 10562
  • [7] Classical theory for second-harmonic generation from metallic nanoparticles
    Zeng, Yong
    Hoyer, Walter
    Liu, Jinjie
    Koch, Stephan W.
    Moloney, Jerome V.
    PHYSICAL REVIEW B, 2009, 79 (23):
  • [8] Second-harmonic generation in metallic nanoparticles: Clarification of the role of the surface
    Ciraci, Cristian
    Poutrina, Ekaterina
    Scalora, Michael
    Smith, David R.
    PHYSICAL REVIEW B, 2012, 86 (11)
  • [9] Optical second harmonic generation from silicon with embedded silver nanostructures
    Bhowmik, Gourav
    An, Yong Q.
    Diebold, Alain C.
    Huang, Mengbing
    NANOPHOTONIC MATERIALS XV, 2018, 10720
  • [10] Sensitivity of gold nanoparticles Second Harmonic scattering to surrounding medium change
    Nadolski, Krzysztof
    Jonin, Christian
    Salmon, Estelle
    Behel, Zacharie
    Matczyszyn, Katarzyna
    Brevet, Pierre-Francois
    JOURNAL OF MOLECULAR LIQUIDS, 2023, 388
12345