Photoelectric Properties of Planar and Mesoporous Structured Perovskite Solar Cells

被引：11

作者：

Asmontas, Steponas ^{[1
]}

Cerskus, Aurimas ^{[1
]}

Gradauskas, Jonas ^{[1
]}

Griguceviciene, Asta ^{[1
]}

Juskenas, Remigijus ^{[1
]}

Leinartas, Konstantinas ^{[1
]}

Lucun, Andzej ^{[1
]}

Petrauskas, Kazimieras ^{[1
]}

Selskis, Algirdas ^{[1
]}

Staisiunas, Laurynas ^{[1
]}

Suziedelis, Algirdas ^{[1
]}

Silenas, Aldis ^{[1
]}

Sirmulis, Edmundas ^{[1
]}

机构：

[1] Ctr Phys Sci & Technol, Savanoriu Ave 231, LT-02300 Vilnius, Lithuania

来源：

MATERIALS | 2022年 / 15卷 / 12期

关键词：

advanced energy materials; perovskite; solar cell; thin film; power conversion efficiency; EXCITATION-POWER DEPENDENCE; EFFICIENT; PHOTOLUMINESCENCE; LAYER; TIO2; MOBILITIES; LIFETIMES; DYNAMICS; CARRIERS; EDGE;

D O I：

10.3390/ma15124300

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The high efficiency of perovskite solar cells strongly depends on the quality of perovskite films and carrier extraction layers. Here, we present the results of an investigation of the photoelectric properties of solar cells based on perovskite films grown on compact and mesoporous titanium dioxide layers. Kinetics of charge carrier transport and their extraction in triple-cation perovskite solar cells were studied by using transient photovoltage and time-resolved photoluminescence decay measurements. X-ray diffraction analysis revealed that the crystallinity of the perovskite films grown on mesoporous titanium dioxide is better compared to the films grown on compact TiO2. Mesoporous structured perovskite solar cells are found to have higher power conversion efficiency mainly due to enlarged perovskite/mesoporous -TiO2 interfacial area and better crystallinity of their perovskite films.

引用

页数：14

共 47 条

[1] Impact of Cesium Concentration on Optoelectronic Properties of Metal Halide Perovskites [J].

Asmontas, Steponas ;

Cerskus, Aurimas ;

Gradauskas, Jonas ;

Griguceviciene, Asta ;

Juskenas, Remigijus ;

Leinartas, Konstantinas ;

Lucun, Andzej ;

Petrauskas, Kazimieras ;

Selskis, Algirdas ;

Suziedelis, Algirdas ;

Sirmulis, Edmundas .

MATERIALS, 2022, 15 (05)

[2] Cesium-Containing Triple Cation Perovskite Solar Cells [J].

Asmontas, Steponas ;

Cerskus, Aurimas ;

Gradauskas, Jonas ;

Griguceviciene, Asta ;

Leinartas, Konstantinas ;

Lucun, Andzej ;

Petrauskas, Kazimieras ;

Selskis, Algirdas ;

Suziedelis, Algirdas ;

Sirmulis, Edmundas ;

Juskenas, Remigijus .

COATINGS, 2021, 11 (03) :1-12

[3] Low Resistance TiO2/p-Si Heterojunction for Tandem Solar Cells [J].

Asmontas, Steponas ;

Anbinderis, Maksimas ;

Gradauskas, Jonas ;

Juskenas, Remigijus ;

Leinartas, Konstantinas ;

Lucun, Andzej ;

Selskis, Algirdas ;

Staisiunas, Laurynas ;

Stanionyte, Sandra ;

Suziedelis, Algirdas ;

Silenas, Aldis ;

Sirmulis, Edmundas .

MATERIALS, 2020, 13 (12) :1-10

[4] Photoluminescence properties of CdTe/CdTeSe/CdSe core/alloyed/shell type-II quantum dots [J].

Ca, N. X. ;

Hien, N. T. ;

Luyen, N. T. ;

Lien, V. T. K. ;

Thanh, L. D. ;

Do, P., V ;

Bau, N. Q. ;

Pham, T. T. .

JOURNAL OF ALLOYS AND COMPOUNDS, 2019, 787 :823-830

[5] Organometallic Halide Perovskites: Sharp Optical Absorption Edge and Its Relation to Photovoltaic Performance [J].

De Wolf, Stefaan ;

Holovsky, Jakub ;

Moon, Soo-Jin ;

Loeper, Philipp ;

Niesen, Bjoern ;

Ledinsky, Martin ;

Haug, Franz-Josef ;

Yum, Jun-Ho ;

Ballif, Christophe .

JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2014, 5 (06) :1035-1039

[6] Electron-hole diffusion lengths > 175 μm in solution-grown CH3NH3PbI3 single crystals [J].

Dong, Qingfeng ;

Fang, Yanjun ;

Shao, Yuchuan ;

Mulligan, Padhraic ;

Qiu, Jie ;

Cao, Lei ;

Huang, Jinsong .

SCIENCE, 2015, 347 (6225) :967-970

[7] Efficient Photon Recycling and Radiation Trapping in Cesium Lead Halide Perovskite Waveguides [J].

Dursun, Ibrahim ;

Zheng, Yangzi ;

Guo, Tianle ;

De Bastiani, Michele ;

Turedi, Bekir ;

Sinatra, Lutfan ;

Hague, Md Azimul ;

Sun, Bin ;

Zhumekenov, Ayan A. ;

Saidaminov, Makhsud I. ;

de Arquer, F. Pelayo Garcia ;

Sargent, Edward H. ;

Wu, Tom ;

Gartstein, Yuri N. ;

Bakr, Osman M. ;

Mohammed, Omar F. ;

Malko, Anton V. .

ACS ENERGY LETTERS, 2018, 3 (07) :1492-1498

[8] The light and shade of perovskite solar cells [J].

Graetzel, Michael .

NATURE MATERIALS, 2014, 13 (09) :838-842

[9] Revealing the charge carrier kinetics in perovskite solar cells affected by mesoscopic structures and defect states from simple transient photovoltage measurements [J].

Hidayat, Rahmat ;

Nurunnizar, Adhita Asma ;

Fariz, Alvin ;

Herman ;

Rosa, Erlyta Septa ;

Shobih ;

Oizumi, Tomohisa ;

Fujii, Akihiko ;

Ozaki, Masanori .

SCIENTIFIC REPORTS, 2020, 10 (01)

[10] Atomic Layer Deposition of TiO2 for a High-Efficiency Hole-Blocking Layer in Hole-Conductor-Free Perovskite Solar Cells Processed in Ambient Air [J].

Hu, Hang ;

Dong, Binghai ;

Hu, Huating ;

Chen, Fengxiang ;

Kong, Mengqin ;

Zhang, Quping ;

Luo, Tianyue ;

Zhao, Li ;

Guo, Zhiguang ;

Li, Jing ;

Xu, Zuxun ;

Wang, Shimin ;

Eder, Dominik ;

Wan, Li .

ACS APPLIED MATERIALS & INTERFACES, 2016, 8 (28) :17999-18007

← 1 2 3 4 5 →