Spatial Distribution, Environmental Risk and Safe Utilization Zoning of Soil Heavy Metals in Farmland, Subtropical China

被引:17
作者
Guo, Weiwei [1 ]
Wu, Tao [1 ]
Jiang, Guojun [1 ]
Pu, Lijie [2 ]
Zhang, Jianzhen [1 ]
Xu, Fei [3 ]
Yu, Hongmei [1 ]
Xie, Xuefeng [1 ,4 ]
机构
[1] Zhejiang Normal Univ, Coll Geog & Environm Sci, Jinhua 321004, Zhejiang, Peoples R China
[2] Nanjing Univ, Sch Geog & Ocean Sci, Nanjing 210023, Peoples R China
[3] Zhejiang Univ Finance & Econ, Inst Land & Urban Rural Dev, Hangzhou 310018, Peoples R China
[4] Minist Nat Resources, Key Lab Coastal Zone Exploitat & Protect, Nanjing 210023, Peoples R China
基金
中国国家自然科学基金;
关键词
soil heavy metals; spatial variability; environmental risks; safe utilization zoning; YANGTZE-RIVER DELTA; AGRICULTURAL SOILS; SOURCE APPORTIONMENT; POLLUTION INDEXES; HOT-SPOTS; CONTAMINATION; MULTIVARIATE; BALANCE; AREA; INVENTORY;
D O I
10.3390/land10060569
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Heavy metal (HM) accumulation in farmland soil can be transferred to the human body through the food chain, posing a serious threat to human health. Exploring the environmental risk and safe utilization zoning of soil HMs in farmland can provide the basis for the formulation of effective control strategies. Soil samples from typical subtropical farmland were collected in Jinhua City and analyzed for HMs (As, Cd, Cr, Cu, Hg, Ni, Pb, and Zn). The objective of this study was to explore the spatial distribution and environmental risk of soil HMs, and then divide the safe utilization area of soil HMs of farmland in Jinhua City. The results showed that the mean concentrations of soil HMs were, in descending order: Zn (76.05 mg kg(-1)) > Cr (36.73 mg kg(-1)) > Pb (32.48 mg kg(-1)) > Cu (18.60 mg kg(-1)) > Ni (11.95 mg kg(-1)) > As (6.37 mg kg(-1)) > Cd (0.18 mg kg(-1)) > Hg (0.11 mg kg(-1)), and all determined soil HMs did not exceed the risk screening values for soil contamination of agricultural land of China. The fitted semi-variogram showed that the spatial autocorrelation of Cd, Hg, Pb, and Zn was weak, with island-shaped distribution, while As, Cr, Cu, and Ni had medium spatial autocorrelation, with strip-shaped and island-shaped distribution. The hot spot analysis and environmental risk probability showed that the environmental risks of As, Cd, Cu, Pb, Zn, and Cu were relatively high, whereas those of Cr, Hg, and Ni were relatively low. Safe utilization zones and basic safe utilization zones accounted for 89.35% and 8.58% of the total farmland area in Jinhua, respectively, and only a small part of the farmland soil was at risk of use.
引用
收藏
页数:13
相关论文
共 57 条
[41]   Water balance creates a threshold in soil pH at the global scale [J].
Slessarev, E. W. ;
Lin, Y. ;
Bingham, N. L. ;
Johnson, J. E. ;
Dai, Y. ;
Schimel, J. P. ;
Chadwick, O. A. .
NATURE, 2016, 540 (7634) :567-+
[42]   Multivariate and geostatistical analyses of the spatial distribution and sources of heavy metals in agricultural soil in Dehui, Northeast China [J].
Sun, Chongyu ;
Liu, Jingshuang ;
Wang, Yang ;
Sun, Liqiang ;
Yu, Hongwen .
CHEMOSPHERE, 2013, 92 (05) :517-523
[43]   Concentrations, Distribution, and Ecological Risk Assessment of Heavy Metals in Daya Bay, China [J].
Tang, Huijuan ;
Ke, Zhixin ;
Yan, Muting ;
Wang, Wenjing ;
Nie, Huayue ;
Li, Boxing ;
Zhang, Jingping ;
Xu, Xiangrong ;
Wang, Jun .
WATER, 2018, 10 (06)
[44]   Evaluating the probability of exceeding a site-specific soil cadmium contamination threshold [J].
Van Meirvenne, M ;
Goovaerts, P .
GEODERMA, 2001, 102 (1-2) :75-100
[45]   Assessment of heavy metal contamination in sediments of the Tigris River (Turkey) using pollution indices and multivariate statistical techniques [J].
Varol, Memet .
JOURNAL OF HAZARDOUS MATERIALS, 2011, 195 :355-364
[46]  
Wang Fei, 2016, Huanjing Kexue, V37, P3144, DOI [10.13227/j.hjkx.2016.08.041, 10.13277/j.hjkx.2016.08.041]
[47]  
[汪庆华 WANG Qinghua], 2007, [地质通报, Geological Bulletin of China], V26, P590
[48]   Spatial distribution and source apportionment of heavy metals in soil from a typical county-level city of Guangdong Province, China [J].
Wang, Shuo ;
Cai, Li-Mei ;
Wen, Han-Hui ;
Luo, Jie ;
Wang, Qiu-Shuang ;
Liu, Xie .
SCIENCE OF THE TOTAL ENVIRONMENT, 2019, 655 :92-101
[49]   Risk assessment for and microbial community changes in Farmland soil contaminated with heavy metals and metalloids [J].
Wang, Xu ;
Gao, Ping ;
Li Daping ;
Liu, Ju ;
Yang, Nuan ;
Gu, Wenzhi ;
He, Xiaohong ;
Tang, Wenzhong .
ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY, 2019, 185
[50]   A review of heavy metal contaminations in urban soils, urban road dusts and agricultural soils from China [J].
Wei, Binggan ;
Yang, Linsheng .
MICROCHEMICAL JOURNAL, 2010, 94 (02) :99-107